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@ARTICLE{Jiang:904167,
      author       = {Jiang, Ming and Zhang, Qian and Danilov, Dmitri and Eichel,
                      Rüdiger-A. and Notten, Peter H. L.},
      title        = {{F}ormation of a {S}table {S}olid-{E}lectrolyte
                      {I}nterphase at {M}etallic {L}ithium {A}nodes {I}nduced by
                      {L}i{N}b{O} 3 {P}rotective {L}ayers},
      journal      = {ACS applied energy materials},
      volume       = {4},
      number       = {9},
      issn         = {2574-0962},
      address      = {Washington, DC},
      publisher    = {ACS Publications},
      reportid     = {FZJ-2021-05737},
      pages        = {10333 - 10343},
      year         = {2021},
      abstract     = {The stability of solid-electrolyte interphase (SEI) surface
                      films at Li-metal anodes is crucial for the safe and durable
                      operation of lithium-metal batteries (LMBs). By combining
                      Li-metal anodes with high-performance Ni-rich
                      transition-metal oxide cathodes, LMBs can meet the goal of a
                      high specific energy density of more than 500 Wh kg–1.
                      However, Li-metal anodes suffer from serious problems,
                      especially the nonuniform lithium deposition and
                      uncontrollable SEI formation. In this work, Li-metal anodes
                      were protected by thin-film LiNbO3 coatings. Full cells
                      composed of protected Li-metal anodes and
                      LiNi0.6Co0.2Mn0.2O2 cathodes were examined electrochemically
                      and by physical characterization methods. Postmortem
                      analyses of pristine and prolonged cycled Li-metal anodes
                      were performed. The results revealed the formation of more
                      stable SEI films at the protected Li-metal anodes in
                      comparison to unprotected electrodes. Consequently, the
                      LiNbO3 layers improved the cycle-life performance of
                      Li-metal anodes in LMBs. Furthermore, X-ray photoelectron
                      spectroscopy (XPS) analyses showed that the reduction of
                      metallic ions stemming from the Ni-rich cathodes was also
                      inhibited by the protective LiNbO3 layers, thereby further
                      controlling the degradation of Li-metal anodes.},
      cin          = {IEK-9},
      ddc          = {540},
      cid          = {I:(DE-Juel1)IEK-9-20110218},
      pnm          = {1223 - Batteries in Application (POF4-122)},
      pid          = {G:(DE-HGF)POF4-1223},
      typ          = {PUB:(DE-HGF)16},
      UT           = {WOS:000703338600168},
      doi          = {10.1021/acsaem.1c02278},
      url          = {https://juser.fz-juelich.de/record/904167},
}