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@ARTICLE{Liu:904175,
      author       = {Liu, Xiangsi and Liang, Ziteng and Xiang, Yuxuan and Lin,
                      Min and Li, Qi and Liu, Zigeng and Zhong, Guiming and Fu,
                      Riqiang and Yang, Yong},
      title        = {{S}olid‐{S}tate {NMR} and {MRI} {S}pectroscopy for
                      {L}i/{N}a {B}atteries: {M}aterials, {I}nterface, and {I}n
                      {S}itu {C}haracterization},
      journal      = {Advanced materials},
      volume       = {33},
      number       = {50},
      issn         = {0935-9648},
      address      = {Weinheim},
      publisher    = {Wiley-VCH},
      reportid     = {FZJ-2021-05745},
      pages        = {2005878 -},
      year         = {2021},
      abstract     = {Enhancing the electrochemical performance of batteries,
                      including the lifespan, energy, and power densities, is an
                      everlasting quest for the rechargeable battery community.
                      However, the dynamic and coupled (electro)chemical processes
                      that occur in the electrode materials as well as at the
                      electrode/electrolyte interfaces complicate the
                      investigation of their working and decay mechanisms. Herein,
                      the recent developments and applications of solid-state
                      nuclear magnetic resonance (ssNMR) and magnetic resonance
                      imaging (MRI) techniques in Li/Na batteries are reviewed.
                      Several typical cases including the applications of NMR
                      spectroscopy for the investigation of the pristine structure
                      and the dynamic structural evolution of materials are first
                      emphasized. The NMR applications in analyzing the solid
                      electrolyte interfaces (SEI) on the electrode are further
                      concluded, involving the identification of SEI components
                      and investigation of ionic motion through the interfaces.
                      Beyond, the new development of in situ NMR and MRI
                      techniques are highlighted, including their advantages,
                      challenges, applications and the design principle of in situ
                      cell. In the end, a prospect about how to use ssNMR in
                      battery research from the perspectives of materials,
                      interface, and in situ NMR, aiming at obtaining deeper
                      insight of batteries with the assistance of ssNMR is
                      represented.},
      cin          = {IEK-9},
      ddc          = {660},
      cid          = {I:(DE-Juel1)IEK-9-20110218},
      pnm          = {1232 - Power-based Fuels and Chemicals (POF4-123)},
      pid          = {G:(DE-HGF)POF4-1232},
      typ          = {PUB:(DE-HGF)16},
      pubmed       = {33788341},
      UT           = {WOS:000635235300001},
      doi          = {10.1002/adma.202005878},
      url          = {https://juser.fz-juelich.de/record/904175},
}