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| 001 | 904180 | ||
| 005 | 20250514114657.0 | ||
| 024 | 7 | _ | |a 10.1002/admi.202100967 |2 doi |
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| 037 | _ | _ | |a FZJ-2021-05750 |
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| 100 | 1 | _ | |a Türk, Hanna |0 P:(DE-HGF)0 |b 0 |
| 245 | _ | _ | |a Complexions at the Electrolyte/Electrode Interface in Solid Oxide Cells |
| 260 | _ | _ | |a Weinheim |c 2021 |b Wiley-VCH |
| 336 | 7 | _ | |a article |2 DRIVER |
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| 520 | _ | _ | |a Rapid deactivation presently limits a wide spread use of high-temperature solid oxide cells (SOCs) as otherwise highly efficient chemical energy converters. With deactivation triggered by the ongoing conversion reactions, an atomic-scale understanding of the active triple-phase boundary between electrolyte, electrode, and gas phase is essential to increase cell performance. Here, a multi-method approach is used comprising transmission electron microscopy and first-principles calculations and molecular simulations to untangle the atomic arrangement of the prototypical SOC interface between a lanthanum strontium manganite (LSM) anode and a yttria-stabilized zirconia (YSZ) electrolyte in the as-prepared state after sintering. An interlayer of self-limited width with partial amorphization and strong compositional gradient is identified, thus exhibiting the characteristics of a complexion that is stabilized by the confinement between two bulk phases. This offers a new perspective to understand the function of SOCs at the atomic scale. Moreover, it opens up a hitherto unrealized design space to tune the conversion efficiency. |
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| 700 | 1 | _ | |a Schmidt, Franz-Philipp |0 P:(DE-HGF)0 |b 1 |
| 700 | 1 | _ | |a Götsch, Thomas |0 P:(DE-HGF)0 |b 2 |e Corresponding author |
| 700 | 1 | _ | |a Girgsdies, Frank |0 P:(DE-HGF)0 |b 3 |
| 700 | 1 | _ | |a Hammud, Adnan |0 P:(DE-HGF)0 |b 4 |
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| 700 | 1 | _ | |a Lunkenbein, Thomas |0 P:(DE-HGF)0 |b 13 |
| 773 | _ | _ | |a 10.1002/admi.202100967 |g Vol. 8, no. 18, p. 2100967 - |0 PERI:(DE-600)2750376-8 |n 18 |p 2100967 - |t Advanced materials interfaces |v 8 |y 2021 |x 2196-7350 |
| 856 | 4 | _ | |u https://juser.fz-juelich.de/record/904180/files/Adv%20Materials%20Inter%20-%202021%20-%20T%20rk%20-%20Complexions%20at%20the%20Electrolyte%20Electrode%20Interface%20in%20Solid%20Oxide%20Cells.pdf |y OpenAccess |
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