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@ARTICLE{Butzelaar:904234,
      author       = {Butzelaar, Andreas J. and Liu, Kun L. and Röring, Philipp
                      and Brunklaus, Gunther and Winter, Martin and Theato,
                      Patrick},
      title        = {{A} {S}ystematic {S}tudy of {V}inyl {E}ther-{B}ased
                      {P}oly({E}thylene {O}xide) {S}ide-{C}hain {P}olymer
                      {E}lectrolytes},
      journal      = {ACS applied polymer materials},
      volume       = {3},
      number       = {3},
      issn         = {2637-6105},
      address      = {Washington, DC},
      publisher    = {ACS Publications},
      reportid     = {FZJ-2021-05804},
      pages        = {1573 - 1582},
      year         = {2021},
      abstract     = {Herein, we report on the synthesis of a systematic library
                      of vinyl ether-based poly(ethylene oxide) (PEO) side-chain
                      copolymers in order to reduce the crystallization of PEO.
                      The influence of different grafted PEO side chain lengths,
                      the grafting density, and the [Li+]:[EO] ratio after mixing
                      with LiTFSI on the glass transition temperature (Tg), the
                      crystallinity, and the resulting ionic conductivity was
                      examined. Copolymers bearing longer PEO side chains and
                      higher grafting densities show higher crystallization
                      tendencies while their Tg is reduced at the same time.
                      Furthermore, the addition of LiTFSI reduces crystallization
                      but increases Tg. Because these effects are directly
                      impacting the ionic conductivity, we demonstrate that the
                      different parameters need to be carefully adjusted in order
                      to balance their influence. In this way, a fundamental view
                      that shows the potential of PEO side-chain copolymers for
                      their applications as polymer electrolytes is provided.},
      cin          = {IEK-12},
      ddc          = {540},
      cid          = {I:(DE-Juel1)IEK-12-20141217},
      pnm          = {1221 - Fundamentals and Materials (POF4-122)},
      pid          = {G:(DE-HGF)POF4-1221},
      typ          = {PUB:(DE-HGF)16},
      UT           = {WOS:000629192800035},
      doi          = {10.1021/acsapm.0c01398},
      url          = {https://juser.fz-juelich.de/record/904234},
}