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@ARTICLE{Huang:904279,
      author       = {Huang, Jun},
      title        = {{S}tatistical {T}reatment of {A}ctivity and {D}urability of
                      {E}lectrocatalysts with {D}istributed {B}inding {E}nergies},
      journal      = {Journal of the Electrochemical Society},
      volume       = {168},
      number       = {6},
      issn         = {0013-4651},
      address      = {Bristol},
      publisher    = {IOP Publishing},
      reportid     = {FZJ-2021-05849},
      pages        = {066507 -},
      year         = {2021},
      abstract     = {We present a statistical treatment of the catalytic
                      activity and durability of nonhomogeneous electrocatalysts
                      that possess distributed binding energies of reaction
                      intermediates. The treatment is simple, generic, and
                      amenable to analytical solutions. It is revealed that the
                      highest overall catalytic activity is obtained with a
                      suitable level of nonhomogeneity that is commensurate with
                      the average property. The evolution of the binding energy
                      distribution is described by the Fokker-Planck theory.
                      Exponential decay of the catalytic activity is predicted
                      theoretically and confirmed experimentally. The exponential
                      decay shows one- or two stages, depending on the initial
                      distribution properties. The present work represents a step
                      toward closing the gap between ideal and practical
                      electrocatalysts using statistical considerations.},
      cin          = {IEK-13},
      ddc          = {660},
      cid          = {I:(DE-Juel1)IEK-13-20190226},
      pnm          = {1231 - Electrochemistry for Hydrogen (POF4-123)},
      pid          = {G:(DE-HGF)POF4-1231},
      typ          = {PUB:(DE-HGF)16},
      UT           = {WOS:000659215800001},
      doi          = {10.1149/1945-7111/ac0362},
      url          = {https://juser.fz-juelich.de/record/904279},
}