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@ARTICLE{Moors:904589,
      author       = {Moors, Marco and An, Yun and Kuc, Agnieszka and Monakhov,
                      Kirill Yu},
      title        = {{T}i{O} x /{P}t 3 {T}i(111) surface-directed formation of
                      electronically responsive supramolecular assemblies of
                      tungsten oxide clusters},
      journal      = {Beilstein journal of nanotechnology},
      volume       = {12},
      issn         = {2190-4286},
      address      = {Frankfurt, M.},
      publisher    = {Beilstein-Institut zur Förderung der Chemischen
                      Wissenschaften},
      reportid     = {FZJ-2021-06159},
      pages        = {203 - 212},
      year         = {2021},
      abstract     = {Highly ordered titanium oxide films grown on a Pt3Ti(111)
                      alloy surface were utilized for the controlled
                      immobilization and tip-induced electric field-triggered
                      electronic manipulation of nanoscopic W3O9 clusters.
                      Depending on the operating conditions, two different stable
                      oxide phases, z’-TiOx and w’-TiOx, were produced. These
                      phases show a strong effect on the adsorption
                      characteristics and reactivity of W3O9 clusters, which are
                      formed as a result of thermal evaporation of WO3 powder on
                      the complex TiOx/Pt3Ti(111) surfaces under ultra-high vacuum
                      conditions. The physisorbed tritungsten nano-oxides were
                      found as isolated single units located on the metallic
                      attraction points or as supramolecular self-assemblies with
                      a W3O9-capped hexagonal scaffold of W3O9 units. By applying
                      scanning tunneling microscopy to the W3O9–(W3O9)6
                      structures, individual units underwent a tip-induced
                      reduction to W3O8. At elevated temperatures, agglomeration
                      and growth of large WO3 islands, which thickness is strongly
                      limited to a maximum of two unit cells, were observed. The
                      findings boost progress toward template-directed nucleation,
                      growth, networking, and charge state manipulation of
                      functional molecular nanostructures on surfaces using
                      operando techniques.},
      cin          = {PGI-7 / JARA-FIT},
      ddc          = {620},
      cid          = {I:(DE-Juel1)PGI-7-20110106 / $I:(DE-82)080009_20140620$},
      pnm          = {5233 - Memristive Materials and Devices (POF4-523)},
      pid          = {G:(DE-HGF)POF4-5233},
      typ          = {PUB:(DE-HGF)16},
      pubmed       = {33728238},
      UT           = {WOS:000618878500001},
      doi          = {10.3762/bjnano.12.16},
      url          = {https://juser.fz-juelich.de/record/904589},
}