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| Hauptseite > Publikationsdatenbank > TiO x /Pt 3 Ti(111) surface-directed formation of electronically responsive supramolecular assemblies of tungsten oxide clusters > print |
| Hauptseite > Publikationsdatenbank > TiO x /Pt 3 Ti(111) surface-directed formation of electronically responsive supramolecular assemblies of tungsten oxide clusters > print |
| 001 | 904589 | ||
| 005 | 20220131120431.0 | ||
| 024 | 7 | _ | |a 10.3762/bjnano.12.16 |2 doi |
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| 037 | _ | _ | |a FZJ-2021-06159 |
| 082 | _ | _ | |a 620 |
| 100 | 1 | _ | |a Moors, Marco |0 P:(DE-Juel1)145323 |b 0 |
| 245 | _ | _ | |a TiO x /Pt 3 Ti(111) surface-directed formation of electronically responsive supramolecular assemblies of tungsten oxide clusters |
| 260 | _ | _ | |a Frankfurt, M. |c 2021 |b Beilstein-Institut zur Förderung der Chemischen Wissenschaften |
| 336 | 7 | _ | |a article |2 DRIVER |
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| 520 | _ | _ | |a Highly ordered titanium oxide films grown on a Pt3Ti(111) alloy surface were utilized for the controlled immobilization and tip-induced electric field-triggered electronic manipulation of nanoscopic W3O9 clusters. Depending on the operating conditions, two different stable oxide phases, z’-TiOx and w’-TiOx, were produced. These phases show a strong effect on the adsorption characteristics and reactivity of W3O9 clusters, which are formed as a result of thermal evaporation of WO3 powder on the complex TiOx/Pt3Ti(111) surfaces under ultra-high vacuum conditions. The physisorbed tritungsten nano-oxides were found as isolated single units located on the metallic attraction points or as supramolecular self-assemblies with a W3O9-capped hexagonal scaffold of W3O9 units. By applying scanning tunneling microscopy to the W3O9–(W3O9)6 structures, individual units underwent a tip-induced reduction to W3O8. At elevated temperatures, agglomeration and growth of large WO3 islands, which thickness is strongly limited to a maximum of two unit cells, were observed. The findings boost progress toward template-directed nucleation, growth, networking, and charge state manipulation of functional molecular nanostructures on surfaces using operando techniques. |
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| 700 | 1 | _ | |a An, Yun |0 P:(DE-HGF)0 |b 1 |
| 700 | 1 | _ | |a Kuc, Agnieszka |0 0000-0002-9458-4136 |b 2 |
| 700 | 1 | _ | |a Monakhov, Kirill Yu |0 P:(DE-Juel1)167441 |b 3 |e Corresponding author |
| 773 | _ | _ | |a 10.3762/bjnano.12.16 |g Vol. 12, p. 203 - 212 |0 PERI:(DE-600)2583584-1 |p 203 - 212 |t Beilstein journal of nanotechnology |v 12 |y 2021 |x 2190-4286 |
| 856 | 4 | _ | |u https://juser.fz-juelich.de/record/904589/files/2190-4286-12-16.pdf |y OpenAccess |
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