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@ARTICLE{Seifert:904679,
      author       = {Seifert, Julian and Günzing, Damian and Webers, Samira and
                      Dulle, Martin and Kruteva, Margarita and Landers, Joachim
                      and Wende, Heiko and Schmidt, Annette M.},
      title        = {{S}train- and field-induced anisotropy in hybrid elastomers
                      with elongated filler nanoparticles},
      journal      = {Soft matter},
      volume       = {17},
      number       = {32},
      issn         = {1744-683X},
      address      = {London},
      publisher    = {Royal Soc. of Chemistry},
      reportid     = {FZJ-2022-00028},
      pages        = {7565 - 7584},
      year         = {2021},
      abstract     = {The implementation of anisotropy to functional materials is
                      a key step towards future smart materials. In this work, we
                      evaluate the influence of preorientation and sample
                      architecture on the strain-induced anisotropy in hybrid
                      elastomers containing covalently attached elongated magnetic
                      filler particles. Accordingly, silica coated spindle-type
                      hematite particles are incorporated to
                      poly(dimethylsiloxane)-based elastomers, and two types of
                      composite architectures are compared: On the one hand a
                      conventional architecture of filled, covalently crosslinked
                      elastomers, and on the other hybrid elastomers that are
                      crosslinked exclusively by covalent attachment of the
                      polymer chains to the particle surface. By the application
                      of external strain and with magnetic fields, the
                      orientational order of the elongated particles can be
                      manipulated, and we investigate the interplay between
                      strain, magnetic order, and orientational order of the
                      particles by combining 2D small angle X-ray scattering
                      experiments under strain and fields with Mössbauer
                      spectroscopy under similar conditions, and supplementary
                      angular-dependent magnetization experiments. The converging
                      information is used to quantify the order in these
                      interesting materials, while establishing a direct link
                      between the magnetic properties and the spatial orientation
                      of the embedded magnetic nanoparticles.},
      cin          = {JCNS-1 / IBI-8},
      ddc          = {530},
      cid          = {I:(DE-Juel1)JCNS-1-20110106 / I:(DE-Juel1)IBI-8-20200312},
      pnm          = {6G4 - Jülich Centre for Neutron Research (JCNS) (FZJ)
                      (POF4-6G4) / 633 - Life Sciences – Building Blocks of
                      Life: Structure and Function (POF4-633) / 5251 - Multilevel
                      Brain Organization and Variability (POF4-525) / 5241 -
                      Molecular Information Processing in Cellular Systems
                      (POF4-524)},
      pid          = {G:(DE-HGF)POF4-6G4 / G:(DE-HGF)POF4-633 /
                      G:(DE-HGF)POF4-5251 / G:(DE-HGF)POF4-5241},
      typ          = {PUB:(DE-HGF)16},
      pubmed       = {34341807},
      UT           = {WOS:000680397600001},
      doi          = {10.1039/D0SM02104K},
      url          = {https://juser.fz-juelich.de/record/904679},
}