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@ARTICLE{Langer:904795,
author = {Langer, Eike M. and Kegler, Philip and Kowalski, Piotr M.
and Wang, Shuao and Alekseev, Evgeny V.},
title = {{A}chieving and {S}tabilizing {U}ranyl {B}ending via
{P}hysical {P}ressure},
journal = {Inorganic chemistry},
volume = {60},
number = {12},
issn = {0020-1669},
address = {Washington, DC},
publisher = {American Chemical Society},
reportid = {FZJ-2022-00125},
pages = {8419 - 8422},
year = {2021},
abstract = {Applying physical pressure in the uranyl–sulfate system
has resulted in the formation of the first purely inorganic
uranyl oxo-salt phase with a considerable uranyl bend:
Na4[(UO2)(SO4)3]. In addition to a strong bend of the
typically almost linear O═U═O, the typically equatorial
plane is broken up by two out-of-plane oxygen positions.
Computational investigations show the origin of the bending
to lie in the applied physical pressure and not in the
electronic influence or steric hindrance. The increase in
pressure onto the system has been shown to increase uranyl
bending. Furthermore, the phase formation is compared with a
reference phase of a similar structure without uranyl
bending, and a transition pressure of 2.5 GPa is predicted,
which is well in agreement with the experimental results.},
cin = {PTJ-TRI / IEK-6 / IEK-13 / IEK-9},
ddc = {540},
cid = {I:(DE-Juel1)PTJ-TRI-20090406 / I:(DE-Juel1)IEK-6-20101013 /
I:(DE-Juel1)IEK-13-20190226 / I:(DE-Juel1)IEK-9-20110218},
pnm = {1221 - Fundamentals and Materials (POF4-122) / 1411 -
Nuclear Waste Disposal (POF4-141) / 1232 - Power-based Fuels
and Chemicals (POF4-123)},
pid = {G:(DE-HGF)POF4-1221 / G:(DE-HGF)POF4-1411 /
G:(DE-HGF)POF4-1232},
typ = {PUB:(DE-HGF)16},
pubmed = {34096717},
UT = {WOS:000664576700009},
doi = {10.1021/acs.inorgchem.1c00644},
url = {https://juser.fz-juelich.de/record/904795},
}