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@ARTICLE{Khn:904877,
      author       = {Kühn, Sebastian P. and Edström, Kristina and Winter,
                      Martin and Cekic-Laskovic, Isidora},
      title        = {{F}ace to {F}ace at the {C}athode {E}lectrolyte
                      {I}nterphase: {F}rom {I}nterface {F}eatures to {I}nterphase
                      {F}ormation and {D}ynamics},
      journal      = {Advanced materials interfaces},
      volume       = {9},
      number       = {8},
      issn         = {2196-7350},
      address      = {Weinheim},
      publisher    = {Wiley-VCH},
      reportid     = {FZJ-2022-00193},
      pages        = {2102078 -},
      year         = {2022},
      abstract     = {Development of high-performing lithium-based batteries
                      inevitably calls for a profound understanding and
                      elucidation of the reactivity at the electrode–liquid
                      electrolyte interface and its impact on the overall
                      performance and safety. The formation, composition,
                      properties, and mechanisms of the cathode electrolyte
                      interphase (CEI) formation and function are still to a large
                      extent unknown for most lithium-based battery materials,
                      whereas the same is well considered for the solid
                      electrolyte interphase on negative electrodes in the
                      literature. In particular, in high voltage regions >4.3 V,
                      the oxidative stability limit of most liquid electrolytes is
                      reached and new mechanisms, involving surface reactivity of
                      the active material beside electrolyte decomposition,
                      contribute to the interfacial reactivity and nature of the
                      CEI. Focusing on lithium-based cell chemistries, this review
                      aims to highlight the impact of the still less understood
                      electrolyte decomposition chemistry, dictated by the nature
                      of its components, as well as the in-depth research on the
                      physicochemical and electrochemical properties of CEI
                      formation and evolution at positive electrode material
                      surface and sub-surfaces.},
      cin          = {IEK-12},
      ddc          = {600},
      cid          = {I:(DE-Juel1)IEK-12-20141217},
      pnm          = {1221 - Fundamentals and Materials (POF4-122)},
      pid          = {G:(DE-HGF)POF4-1221},
      typ          = {PUB:(DE-HGF)16},
      UT           = {WOS:000737073400001},
      doi          = {10.1002/admi.202102078},
      url          = {https://juser.fz-juelich.de/record/904877},
}