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000904945 1001_ $$0P:(DE-HGF)0$$aQi, Rui$$b0
000904945 245__ $$aA highly-stable layered Fe/Mn-based cathode with ultralow strain for advanced sodium-ion batteries
000904945 260__ $$aAmsterdam [u.a.]$$bElsevier$$c2021
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000904945 520__ $$aSodium-ion batteries (SIBs) with iron- and manganese-based cathode electrodes have exhibited great promise in the grid-scale energy storage systems, on the basis of the satisfactory theoretical capacity, as well as huge abundance, low price and non-toxicity of raw materials. However, the inferior cycle life of cathode materials originating from their poor structural stability remains a formidable challenge towards practical applications. Here, an efficient strategy of improving the structure durability is demonstrated in iron- and manganese-based cathodes by dual heteroatom doping. The as-obtained P2-type Na0.65Li0.08Cu0.08Fe0.24Mn0.6O2 cathode delivers superior cyclability (88.2% capacity retention for 500 cycles at 2C), fabulous rate capability (76% capacity retention at 5C compared to 0.1C), and a useable reversible capacity of around 85 mAh g−1 at 0.1C. Through in-depth characterizations, the underlying structure-property relationship is established, revealing that the complete solid-solution reaction during cycling ensures the ultralow volume variation (as small as 0.7%) and excellent electrochemical performance. These results highlight the significance of fabricating a stable host for the design and development of advanced SIBs with long life.
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000904945 7001_ $$0P:(DE-HGF)0$$aChu, Mihai$$b1
000904945 7001_ $$0P:(DE-HGF)0$$aZhao, Wenguang$$b2
000904945 7001_ $$0P:(DE-HGF)0$$aLiao, Lei$$b3
000904945 7001_ $$0P:(DE-HGF)0$$aChen, Ziwei$$b4
000904945 7001_ $$0P:(DE-HGF)0$$aZheng, Shisheng$$b5
000904945 7001_ $$0P:(DE-HGF)0$$aChen, Xiping$$b6
000904945 7001_ $$0P:(DE-HGF)0$$aXie, Lei$$b7
000904945 7001_ $$0P:(DE-HGF)0$$aLiu, Tongchao$$b8
000904945 7001_ $$0P:(DE-HGF)0$$aRen, Yang$$b9
000904945 7001_ $$0P:(DE-Juel1)145711$$aJin, Lei$$b10$$ufzj
000904945 7001_ $$0P:(DE-HGF)0$$aAmine, Khalil$$b11
000904945 7001_ $$0P:(DE-HGF)0$$aPan, Feng$$b12$$eCorresponding author
000904945 7001_ $$0P:(DE-Juel1)131047$$aXiao, Yinguo$$b13$$eCorresponding author
000904945 773__ $$0PERI:(DE-600)2648700-7$$a10.1016/j.nanoen.2021.106206$$gVol. 88, p. 106206 -$$p106206 -$$tNano energy$$v88$$x2211-2855$$y2021
000904945 8564_ $$uhttps://juser.fz-juelich.de/record/904945/files/1.%20A%20highly%20stable-complete.pdf$$yPublished on 2021-05-31. Available in OpenAccess from 2023-05-31.
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