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| Hauptseite > Publikationsdatenbank > A highly-stable layered Fe/Mn-based cathode with ultralow strain for advanced sodium-ion batteries > print |
| Hauptseite > Publikationsdatenbank > A highly-stable layered Fe/Mn-based cathode with ultralow strain for advanced sodium-ion batteries > print |
| 001 | 904945 | ||
| 005 | 20220131120442.0 | ||
| 024 | 7 | _ | |a 10.1016/j.nanoen.2021.106206 |2 doi |
| 024 | 7 | _ | |a 2211-2855 |2 ISSN |
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| 037 | _ | _ | |a FZJ-2022-00259 |
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| 100 | 1 | _ | |a Qi, Rui |0 P:(DE-HGF)0 |b 0 |
| 245 | _ | _ | |a A highly-stable layered Fe/Mn-based cathode with ultralow strain for advanced sodium-ion batteries |
| 260 | _ | _ | |a Amsterdam [u.a.] |c 2021 |b Elsevier |
| 336 | 7 | _ | |a article |2 DRIVER |
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| 336 | 7 | _ | |a Journal Article |0 0 |2 EndNote |
| 520 | _ | _ | |a Sodium-ion batteries (SIBs) with iron- and manganese-based cathode electrodes have exhibited great promise in the grid-scale energy storage systems, on the basis of the satisfactory theoretical capacity, as well as huge abundance, low price and non-toxicity of raw materials. However, the inferior cycle life of cathode materials originating from their poor structural stability remains a formidable challenge towards practical applications. Here, an efficient strategy of improving the structure durability is demonstrated in iron- and manganese-based cathodes by dual heteroatom doping. The as-obtained P2-type Na0.65Li0.08Cu0.08Fe0.24Mn0.6O2 cathode delivers superior cyclability (88.2% capacity retention for 500 cycles at 2C), fabulous rate capability (76% capacity retention at 5C compared to 0.1C), and a useable reversible capacity of around 85 mAh g−1 at 0.1C. Through in-depth characterizations, the underlying structure-property relationship is established, revealing that the complete solid-solution reaction during cycling ensures the ultralow volume variation (as small as 0.7%) and excellent electrochemical performance. These results highlight the significance of fabricating a stable host for the design and development of advanced SIBs with long life. |
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| 700 | 1 | _ | |a Chu, Mihai |0 P:(DE-HGF)0 |b 1 |
| 700 | 1 | _ | |a Zhao, Wenguang |0 P:(DE-HGF)0 |b 2 |
| 700 | 1 | _ | |a Liao, Lei |0 P:(DE-HGF)0 |b 3 |
| 700 | 1 | _ | |a Chen, Ziwei |0 P:(DE-HGF)0 |b 4 |
| 700 | 1 | _ | |a Zheng, Shisheng |0 P:(DE-HGF)0 |b 5 |
| 700 | 1 | _ | |a Chen, Xiping |0 P:(DE-HGF)0 |b 6 |
| 700 | 1 | _ | |a Xie, Lei |0 P:(DE-HGF)0 |b 7 |
| 700 | 1 | _ | |a Liu, Tongchao |0 P:(DE-HGF)0 |b 8 |
| 700 | 1 | _ | |a Ren, Yang |0 P:(DE-HGF)0 |b 9 |
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| 700 | 1 | _ | |a Amine, Khalil |0 P:(DE-HGF)0 |b 11 |
| 700 | 1 | _ | |a Pan, Feng |0 P:(DE-HGF)0 |b 12 |e Corresponding author |
| 700 | 1 | _ | |a Xiao, Yinguo |0 P:(DE-Juel1)131047 |b 13 |e Corresponding author |
| 773 | _ | _ | |a 10.1016/j.nanoen.2021.106206 |g Vol. 88, p. 106206 - |0 PERI:(DE-600)2648700-7 |p 106206 - |t Nano energy |v 88 |y 2021 |x 2211-2855 |
| 856 | 4 | _ | |u https://juser.fz-juelich.de/record/904945/files/1.%20A%20highly%20stable-complete.pdf |y Published on 2021-05-31. Available in OpenAccess from 2023-05-31. |
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