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@ARTICLE{Smolentseva:905009,
author = {Smolentseva, Anastasia and Goncharov, Ivan M. and Yudenko,
Anna and Bogorodskiy, Andrey and Semenov, Oleg and
Nazarenko, Vera V. and Borshchevskiy, Valentin and Fonin,
Alexander V. and Remeeva, Alina and Jaeger, Karl-Erich and
Krauss, Ulrich and Gordeliy, Valentin and Gushchin, Ivan},
title = {{E}xtreme dependence of {C}hloroflexus aggregans {LOV}
domain thermo- and photostability on the bound flavin
species},
journal = {Photochemical $\&$ photobiological sciences},
volume = {20},
number = {12},
issn = {1474-905X},
address = {Cambridge},
publisher = {Royal Society of Chemistry},
reportid = {FZJ-2022-00320},
pages = {1645 - 1656},
year = {2021},
abstract = {Light-oxygen-voltage (LOV) domains are common photosensory
modules that found many applications in fluorescence
microscopy and optogenetics. Here, we show that the
Chloroflexus aggregans LOV domain can bind different flavin
species (lumichrome, LC; riboflavin, RF; flavin
mononucleotide, FMN; flavin adenine dinucleotide, FAD)
during heterologous expression and that its physicochemical
properties depend strongly on the nature of the bound
flavin. We show that whereas the dissociation constants for
different chromophores are similar, the melting temperature
of the protein reconstituted with single flavin species
varies from ~ 60 °C for LC to ~ 81 °C for FMN, and
photobleaching half-times vary almost 100-fold. These
observations serve as a caution for future studies of LOV
domains in non-native conditions yet raise the possibility
of fine-tuning various properties of LOV-based fluorescent
probes and optogenetic tools by manipulating the chromophore
composition.},
cin = {IMET / IBG-1 / IBI-7},
ddc = {620},
cid = {I:(DE-Juel1)IMET-20090612 / I:(DE-Juel1)IBG-1-20101118 /
I:(DE-Juel1)IBI-7-20200312},
pnm = {2171 - Biological and environmental resources for
sustainable use (POF4-217) / 5241 - Molecular Information
Processing in Cellular Systems (POF4-524)},
pid = {G:(DE-HGF)POF4-2171 / G:(DE-HGF)POF4-5241},
typ = {PUB:(DE-HGF)16},
pubmed = {34796467},
UT = {WOS:000720258200001},
doi = {10.1007/s43630-021-00138-3},
url = {https://juser.fz-juelich.de/record/905009},
}