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@INPROCEEDINGS{Wuttig:905428,
author = {Wuttig, Matthias},
title = {{F}unctional {M}aterials by {D}esign:{D}eveloping
{T}reasure {M}aps with {Q}uantum {C}hemistry},
reportid = {FZJ-2022-00669},
year = {2021},
abstract = {Scientists and practitioners have long dreamt of designing
materials with novel properties. Yet, a hundred years after
quantum mechanics lay the foundations for a systematic
description of the properties of solids, it is still not
possible to predict the best material in applications such
as photovoltaics, superconductivity or thermoelectric energy
conversion. This is a sign of the complexity of the problem,
which is often exacerbated by the need to optimize
conflicting material properties. Hence, one can ponder if
design routes for materials can be devised. In recent years,
the focus of our work has been on designing advanced
functional materials with attractive opto-electronic
properties, including phase change materials,
thermoelectrics, photonic switches and materials for
photovoltaics. To reach this goal, one can try to establish
close links between material properties and chemical
bonding. However, until recently it was quite difficult to
adequately quantify chemical bonds. Some developments in the
last decades, such as the quantum theory of atoms in
molecules [1] have provided the necessary tools to describe
bonds in solids quantitatively. Using these tools, it has
been possible to devise a map which separates different
bonding mechanisms [2]. This map can now be employed to
correlate chemical bonding with material properties [3].
Machine learning and property classification demonstrate the
potential of this approach. These insights are subsequently
employed to design phase change as well as thermoelectric
materials [4,5]. Yet, the discoveries presented here also
force us to revisit the concept of chemical bonds and bring
back a history of vivid scientific disputes about ‘the
nature of the chemical bond’.},
month = {Dec},
date = {2021-12-06},
organization = {MRS Fall Meeting, Boston (USA), 6 Dec
2021 - 8 Dec 2021},
subtyp = {Invited},
cin = {PGI-10},
cid = {I:(DE-Juel1)PGI-10-20170113},
pnm = {5233 - Memristive Materials and Devices (POF4-523)},
pid = {G:(DE-HGF)POF4-5233},
typ = {PUB:(DE-HGF)6},
url = {https://juser.fz-juelich.de/record/905428},
}