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@INPROCEEDINGS{MicuBudisteanu:905441,
author = {Micu-Budisteanu and Bucher, Edith and Sitte, Werner and
Berger, Christian and Lenser, Christian and Menzler, Norbert
H.},
title = {{P}reparation and characterization of
{L}a$_{0.8}${C}a$_{0.2}${F}e$_{0.8}${C}o$_{0.2}${O}$_{3-δ}$
as a new air electrode material for solid oxide cells},
reportid = {FZJ-2022-00682},
year = {2021},
abstract = {Preparation and characterization of
La0.8Ca0.2Fe0.8Co0.2O3-δ as a new air electrode material
for solid oxide cellsMario Micu-Budisteanu1, Christian
Berger2, Edith Bucher1, Christian Lenser3, Norbert H.
Menzler3, Werner Sitte11 Chair of Physical Chemistry,
Montanuniversitaet Leoben, Franz-Josef-Straße 18, 8700
Leoben, Austria2 Max Planck Institute for Solid State
Research, Heisenbergstraße 1, 70569 Stuttgart, Germany3
Forschungszentrum Jülich GmbH, Institute of Energy and
Climate Research – Materials Synthesis and Processing
(IEK-1), 52425 Jülich, GermanyPerovskites from the series
(La,Sr)(Co,Fe)O3-δ are mixed ionic and electronic
conductors that are suitable for a broad variety of possible
applications, with cathodes for solid oxide fuel cells
(SOFCs), anodes for solid oxide electrolyser cells (SOECs),
electrochemical gas sensors and catalysts being the most
promising fields of application. However, due to long-term
stability issues, current research efforts are directed
towards development of alternative Sr-free materials.
Recently, high electronic- and good ionic conductivities, as
well as exceptionally fast oxygen exchange kinetics were
demonstrated for La0.8Ca0.2FeO3-δ (LCF82). In the present
work, substitution of this material with cobalt is
investigated with the aim to further improve sintering
activity and electronic conductivity. Therefore,
La0.8Ca0.2Fe0.8Co0.2O3-δ (LCFC8282) was synthesized using a
sol-gel method. XRD confirmed that the material is single
phase. Thermal expansion coefficients (TEC) were determined
as a function of oxygen partial pressure (1×10-3 ≤
pO2/bar ≤ 1) and temperature (600 ≤ T/°C ≤ 1000). In
comparison of LCF82 with LCFC8282, the TEC of the
Co-substituted material is slightly higher with values of
19-23×10- 6 K-1. The electronic conductivity of LCFC8282 is
in the range of 128 ≤ S cm-1 ≤ 145 at 600 ≤ T/°C ≤
800 and pO2=0.1 bar and thus higher than that of LCF82 (~110
S cm-1). First results on the oxygen exchange kinetics of
LCF8282 show high activity towards oxygen reduction.},
month = {Apr},
date = {2021-04-19},
organization = {KERAMIK 2021- 96. Jahrestagung der
Deutschen Keramischen Gesellschaft,
Online (German), 19 Apr 2021 - 21 Apr
2021},
subtyp = {Other},
cin = {IEK-1},
cid = {I:(DE-Juel1)IEK-1-20101013},
pnm = {1231 - Electrochemistry for Hydrogen (POF4-123) /
Development of improved anodes in solid oxide fuel cells for
conversion of synthesis gas from thermo-chemical
gasification of biomass (275388933)},
pid = {G:(DE-HGF)POF4-1231 / G:(GEPRIS)275388933},
typ = {PUB:(DE-HGF)6},
url = {https://juser.fz-juelich.de/record/905441},
}