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@ARTICLE{Huang:905999,
      author       = {Huang, Zhuojun and Choudhury, Snehashis and Paul, Neelima
                      and Thienenkamp, Johannes Helmut and Lennartz, Peter and
                      Gong, Huaxin and Müller-Buschbaum, Peter and Brunklaus,
                      Gunther and Gilles, Ralph and Bao, Zhenan},
      title        = {{E}ffects of {P}olymer {C}oating {M}echanics at
                      {S}olid‐{E}lectrolyte {I}nterphase for {S}tabilizing
                      {L}ithium {M}etal {A}nodes},
      journal      = {Advanced energy materials},
      volume       = {12},
      number       = {5},
      issn         = {1614-6832},
      address      = {Weinheim},
      publisher    = {Wiley-VCH},
      reportid     = {FZJ-2022-01172},
      pages        = {2103187 -},
      year         = {2022},
      abstract     = {Lithium metal batteries are next-generation energy storage
                      devices that rely on the stable electrodeposition of lithium
                      metal during the charging process. The major challenge
                      associated with this battery chemistry is related to the
                      uneven deposition that leads to dendritic growth and poor
                      coulombic efficiency (CE). A promising strategy for
                      addressing this challenge is utilizing a polymer coating on
                      the anodic surface. While several works in the past have
                      evaluated polymer coatings, the requirements for polymer
                      design are still unclear. In this work, the effect of
                      polymer dynamics on lithium metal deposition is specifically
                      investigated. Electrolyte (solvent) blocking
                      perfluoropolyether polymer networks with evenly spaced
                      H-bonding sites of various strengths are designed, resulting
                      in significant differences in the molecular ordering, as
                      analyzed by X-ray scattering measurements. The differences
                      in the H-bonding strength directly impact the mechanical
                      properties of these materials, thus providing a controlled
                      set of samples with a range of polymer dynamics for
                      electrodeposition studies. Finally, a systematic evaluation
                      of the lithium metal electrodeposition quality with these
                      polymers as anodic coating shows that polymers with
                      flowability or faster polymer dynamics exhibit higher CE.
                      These experimental findings provide rational design
                      principles for soft polymer coatings on lithium metal
                      anodes.},
      cin          = {IEK-12},
      ddc          = {050},
      cid          = {I:(DE-Juel1)IEK-12-20141217},
      pnm          = {1221 - Fundamentals and Materials (POF4-122) / 1222 -
                      Components and Cells (POF4-122) / 1223 - Batteries in
                      Application (POF4-122)},
      pid          = {G:(DE-HGF)POF4-1221 / G:(DE-HGF)POF4-1222 /
                      G:(DE-HGF)POF4-1223},
      typ          = {PUB:(DE-HGF)16},
      UT           = {WOS:000732690000001},
      doi          = {10.1002/aenm.202103187},
      url          = {https://juser.fz-juelich.de/record/905999},
}