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@ARTICLE{Diddens:906100,
author = {Diddens, Diddo and Appiah, Williams Agyei and Mabrouk,
Youssef and Heuer, Andreas and Vegge, Tejs and Bhowmik,
Arghya},
title = {{M}odeling the {S}olid {E}lectrolyte {I}nterphase:
{M}achine {L}earning as a {G}ame {C}hanger?},
journal = {Advanced materials interfaces},
volume = {9},
number = {8},
issn = {2196-7350},
address = {Weinheim},
publisher = {Wiley-VCH},
reportid = {FZJ-2022-01222},
pages = {2101734 -},
year = {2022},
abstract = {The solid electrolyte interphase (SEI) is a complex
passivation layer that forms in situ on many battery
electrodes such as lithium-intercalated graphite or lithium
metal anodes. Its essential function is to prevent the
electrolyte from continuous electrochemical degradation,
while simultaneously allowing ions to pass through, thus
constituting an electronically insulating, but ionically
conducting material. Its properties crucially affect the
overall performance and aging of a battery cell. Despite
decades of intense research, understanding the SEI's precise
formation mechanism, structure, composition, and evolution
remains a conundrum. State-of-the-art computational modeling
techniques are powerful tools to gain additional insights,
although confronted with a trade-off between accuracy and
accessible time- and length scales. In this review, it is
discussed how recent advances in data-driven models,
especially the development of fast and accurate surrogate
simulators and deep generative models, can work with
physics-based and physics-informed approaches to enable the
next generation of breakthroughs in this field. Machine
learning-enhanced multiscale models can provide new pathways
to inverse the design of interphases with desired
properties.},
cin = {IEK-12},
ddc = {600},
cid = {I:(DE-Juel1)IEK-12-20141217},
pnm = {1221 - Fundamentals and Materials (POF4-122)},
pid = {G:(DE-HGF)POF4-1221},
typ = {PUB:(DE-HGF)16},
UT = {WOS:000749645800001},
doi = {10.1002/admi.202101734},
url = {https://juser.fz-juelich.de/record/906100},
}