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| 001 | 906202 | ||
| 005 | 20230123110558.0 | ||
| 024 | 7 | _ | |a 10.1021/acs.jpcc.1c10625 |2 doi |
| 024 | 7 | _ | |a 1932-7447 |2 ISSN |
| 024 | 7 | _ | |a 1932-7455 |2 ISSN |
| 024 | 7 | _ | |a 2128/32208 |2 Handle |
| 024 | 7 | _ | |a WOS:000766228300023 |2 WOS |
| 037 | _ | _ | |a FZJ-2022-01290 |
| 082 | _ | _ | |a 530 |
| 100 | 1 | _ | |a Kraus, Stefan |0 P:(DE-HGF)0 |b 0 |e Corresponding author |
| 245 | _ | _ | |a Uniaxially Aligned 1D Sandwich-Molecular Wires: Electronic Structure and Magnetism |
| 260 | _ | _ | |a Washington, DC |c 2022 |b Soc. |
| 336 | 7 | _ | |a article |2 DRIVER |
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| 520 | _ | _ | |a Sandwich-molecular wires consisting of europium and cyclooctatetraene (Cot) were grown in situ on the moiré of graphene with Ir(110). The moiré templates a uniaxial alignment of monolayer EuCot nanowire carpets and multilayer films with the EuCot wire axis along the [001] direction of the Ir substrate. Using angle-resolved photoemission spectroscopy, we investigate the band structure of the wire carpet films. While π-derived bands were not observed experimentally, we find a flat band 1.85 eV below the Fermi energy. Using density-functional theory and X-ray photoelectron spectroscopy and replacing europium through barium in the sandwich-molecular wires, it is concluded that the flat band is derived from Eu 4f states weakly mixed with Eu 5d states and slightly overlapping with Cot π states. X-ray magnetic circular dichroism is employed to characterize the magnetic properties of the EuCot wire carpet films at low temperatures. Clear evidence for an easy-axis magnetization along the wires is found. |
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| 700 | 1 | _ | |a Herman, Alexander |0 P:(DE-HGF)0 |b 1 |
| 700 | 1 | _ | |a Huttmann, Felix |0 P:(DE-HGF)0 |b 2 |
| 700 | 1 | _ | |a Bianchi, Marco |0 P:(DE-HGF)0 |b 3 |
| 700 | 1 | _ | |a Stan, Raluca-Maria |0 P:(DE-HGF)0 |b 4 |
| 700 | 1 | _ | |a Holt, Ann Julie |0 P:(DE-HGF)0 |b 5 |
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| 700 | 1 | _ | |a Wende, Heiko |0 0000-0001-8395-3541 |b 11 |
| 700 | 1 | _ | |a Hofmann, Philip |0 0000-0002-7367-5821 |b 12 |
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| 700 | 1 | _ | |a Michely, Thomas |0 P:(DE-HGF)0 |b 14 |
| 773 | _ | _ | |a 10.1021/acs.jpcc.1c10625 |g p. acs.jpcc.1c10625 |0 PERI:(DE-600)2256522-X |n 6 |p 3140–3150 |t The journal of physical chemistry |v 126 |y 2022 |x 1932-7447 |
| 856 | 4 | _ | |y Published on 2022-02-07. Available in OpenAccess from 2023-02-07. |u https://juser.fz-juelich.de/record/906202/files/EuCotGrIr110_Manuscript_resub_tm.pdf |
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