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@ARTICLE{Liu:906948,
author = {Liu, Yang and Wilkner, Kai and Unije, Unoaku Victoria and
Baumann, Stefan and Mücke, Robert and Schulze-Küppers,
Falk and Guillon, Olivier},
title = {{P}erformance study of asymmetric oxygen transport
membranes with vertically channelled pores by phase
inversion tape casting},
journal = {Open ceramics},
volume = {9},
issn = {2666-5395},
address = {Amsterdam},
publisher = {Elsevier},
reportid = {FZJ-2022-01766},
pages = {100248 -},
year = {2022},
abstract = {Asymmetric oxygen transport membranes have been extensively
studied revealing the importance of the support porosity. In
this study, asymmetric membranes with vertically channelled
pores were prepared from
Ba0.5Sr0.5(Co0.8Fe0.2)0.97Zr0.03O3-δ (BSCF-Z) by phase
inversion tape casting. The rate-limiting effects of the
membrane layer thickness, the support structure, and the
activation layers were thoroughly analysed. This entails
comparing the permeation rate of the samples with the
membrane layer on different sides of the channelled
supports. Pore tortuosity and computed permeability were
evaluated from 3D-X-ray computed tomography and compared to
previously reported asymmetric membranes prepared by
tape-casting and freeze-drying. Due to a lower pore
tortuosity, the channelled supports have an advantage in gas
transport over the tape cast and freeze cast supports.
However, this is compensated by a thicker membrane layer
(∼54 μm) resulting in similar performance compared to the
thinner membrane layers (∼20 μm) with freeze cast and
tape cast supports.},
cin = {IEK-1},
ddc = {600},
cid = {I:(DE-Juel1)IEK-1-20101013},
pnm = {1232 - Power-based Fuels and Chemicals (POF4-123)},
pid = {G:(DE-HGF)POF4-1232},
typ = {PUB:(DE-HGF)16},
UT = {WOS:001103381000002},
doi = {10.1016/j.oceram.2022.100248},
url = {https://juser.fz-juelich.de/record/906948},
}