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@ARTICLE{Reissig:907018,
      author       = {Reissig, Friederike and Puls, Sebastian and Placke, Tobias
                      and Winter, Martin and Schmuch, Richard and Gómez Martín,
                      Aurora},
      title        = {{I}nvestigation of {L}ithium {P}olyacrylate {B}inders for
                      {A}queous {P}rocessing of {N}i‐{R}ich {L}ithium {L}ayered
                      {O}xide {C}athodes for {L}ithium {I}on {B}atteries},
      journal      = {ChemSusChem},
      volume       = {15},
      number       = {11},
      issn         = {1864-5631},
      address      = {Weinheim},
      publisher    = {Wiley-VCH},
      reportid     = {FZJ-2022-01814},
      pages        = {e202200401},
      year         = {2022},
      abstract     = {Ni-rich layered oxide cathodes are promising candidates to
                      satisfy the increasing energy demand of lithium ion
                      batteries for automotive applications. Aqueous processing of
                      such materials, although being desirable to reduce costs and
                      improve sustainability, remains challenging due to the Li +
                      /H + -exchange upon contact with water, resulting in a pH
                      increase and corrosion of the aluminum current collector.
                      Herein, an example for tuning the properties of aqueous LiNi
                      0.83 Co 0.12 Mn 0.05 O 2 electrode pastes using a lithium
                      polyacrylate-based binder to find the “sweet spot” for
                      processing parameters and electrochemical performance is
                      given. Polyacrylic acid is partially neutralized to balance
                      high initial capacity, good cycling stability and the
                      prevention of aluminum corrosion. Optimized LiOH/polyacrylic
                      acid ratios in water are identified, showing comparable
                      cycling performance to electrodes processed with
                      polyvinylidene difluoride requiring toxic
                      N-methyl-2-pyrrolidone as solvent. This work gives an
                      exemplary study for tuning aqueous electrode pastes
                      properties aiming towards a more environmentally friendly
                      processing of Ni-rich cathodes.},
      cin          = {IEK-12},
      ddc          = {540},
      cid          = {I:(DE-Juel1)IEK-12-20141217},
      pnm          = {1221 - Fundamentals and Materials (POF4-122)},
      pid          = {G:(DE-HGF)POF4-1221},
      typ          = {PUB:(DE-HGF)16},
      pubmed       = {pmid:35333434},
      UT           = {WOS:000789879400001},
      doi          = {10.1002/cssc.202200401},
      url          = {https://juser.fz-juelich.de/record/907018},
}