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000907171 1001_ $$0P:(DE-Juel1)172676$$aLeonard, Kwati$$b0$$eCorresponding author
000907171 245__ $$aAnode supported planar 5 × 5 cm2 SrZr0.5Ce0.4Y0.1O2.95 based solid oxide protonic fuel cells via sequential tape-casting
000907171 260__ $$aAmsterdam [u.a.]$$bElsevier Science$$c2022
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000907171 520__ $$aSolid oxide protonic fuel cells are one of the most efficient means of directly converting stored chemical energy to usable electrical energy. Acceptor-doped Ba(Zr, Ce)O3 perovskite-type oxides are the preferred electrolyte choice as they provide higher conductivity due to lower activation energy. While substantial progress has been made on small-sized protonic laboratory-scale cells, a considerable challenge has been upscaling robust planar-type devices. This paper employs a cost-effective inverse tape casting route and screen printing to fabricate flat planar anode-supported protonic fuel cells consisting of NiO-SrZr0.5Ce0.4Y0.1O3-δ substrate, SrZr0.5Ce0.4Y0.1O3-δ electrolyte, and BaCo0.4Fe0.4Zr0.1Y 0.1O3-δ as the cathode. The processing parameters were analyzed and adjusted to obtain defect-free single cells of dimension up to 100 mm × 100 mm × 0.5 mm with diminished warping. In addition, the smooth tri-layered green tapes yielded suitably dense and gas-tight electrolyte layers after co-sintering at 1300 °C/5 h. Finally, the electrochemical performance of the 50 × 50 mm2 SrZr0.5Ce0.4Y0.1O2.95 based cells was evaluated, and their impedance spectra were deconvoluted to identify all performance-related polarization processes via the distribution of relaxation time.
000907171 536__ $$0G:(DE-HGF)POF4-1232$$a1232 - Power-based Fuels and Chemicals (POF4-123)$$cPOF4-123$$fPOF IV$$x0
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000907171 7001_ $$0P:(DE-Juel1)129617$$aIvanova, Mariya E.$$b1$$ufzj
000907171 7001_ $$0P:(DE-HGF)0$$aWeber, André$$b2
000907171 7001_ $$0P:(DE-Juel1)144923$$aDeibert, Wendelin$$b3$$ufzj
000907171 7001_ $$0P:(DE-Juel1)129637$$aMeulenberg, Wilhelm A.$$b4$$ufzj
000907171 7001_ $$0P:(DE-HGF)0$$aIshihara, Tatsumi$$b5
000907171 7001_ $$0P:(DE-HGF)0$$aMatsumoto, Hiroshige$$b6
000907171 773__ $$0PERI:(DE-600)1500750-9$$a10.1016/j.ssi.2022.115918$$gVol. 379, p. 115918 -$$p115918 -$$tSolid state ionics$$v379$$x0167-2738$$y2022
000907171 8564_ $$uhttps://juser.fz-juelich.de/record/907171/files/1-s2.0-S0167273822000674-main.pdf$$yRestricted
000907171 8564_ $$uhttps://juser.fz-juelich.de/record/907171/files/Manuscript%20file.pdf$$yPublished on 2022-04-07. Available in OpenAccess from 2024-04-07.
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