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@ARTICLE{Wei:907341,
author = {Wei, Jing and Zhang, Xinying and Xia, Longlong and Yuan,
Wenping and Zhou, Zhanyan and Brüggemann, Nicolas},
title = {{R}ole of chemical reactions in the nitrogenous trace gas
emissions and nitrogen retention: {A} meta-analysis},
journal = {The science of the total environment},
volume = {808},
issn = {0048-9697},
address = {Amsterdam [u.a.]},
publisher = {Elsevier Science},
reportid = {FZJ-2022-01976},
pages = {152141 -},
year = {2022},
abstract = {Increasing evidence has been found that chemical reactions
affect significantly the terrestrial nitrogen (N) cycle,
which was previously assumed to be mainly dominated by
biological processes. Due to the limitation of knowledge and
analytical techniques, it is currently challenging to
discern the contribution of biotic and abiotic processes to
the terrestrial N cycle for geobiologists and biogeochemists
alike. To better understand the role of abiotic reactions in
the terrestrial N cycle, it is necessary to comprehend the
chemical controls on nitrogenous trace gas emissions and N
retention in soil under various environmental conditions. In
this manuscript, we assess the role of abiotic reactions in
nitrous oxide (N2O) and nitric oxide (NO) emissions as well
as N retention through a meta-analysis using all related
peer-reviewed publications before August 2020. Results show
that abiotic reactions contributed $29.3–37.7\%$ and
$44.0–57.0\%$ to the total N2O emission and N retention,
representing 3.7–4.7 and 4.0–6.0 Tg year−1 of
global terrestrial N2O emission and N retention,
respectively. Much higher NO production was observed in
sterilized soils than that in unsterilized treatments
indicating the major contribution of chemical reactions to
NO emission and rapid microbial reduction of NO to N2O and
N2. Chemical hydroxylamine oxidation accounts for the
largest abiotic contribution to N2O emission, while chemical
nitrite reduction and fixation represent for the largest
contribution to abiotic NO production and soil N retention,
respectively. Factors influencing the abiotic processes
include pH, total organic carbon (TOC), total nitrogen (TN),
the ratio of carbon to nitrogen (C/N), and transition
metals. These results broadened our knowledge about the
mechanisms involved in chemical N reactions and provided a
simplified estimation about their contribution to
nitrogenous trace gas emission and N retention, which is
meaningful to further study interactions of biologically and
chemically mediated reactions in biogeochemical N cycle.},
cin = {IBG-3},
ddc = {610},
cid = {I:(DE-Juel1)IBG-3-20101118},
pnm = {2173 - Agro-biogeosystems: controls, feedbacks and impact
(POF4-217)},
pid = {G:(DE-HGF)POF4-2173},
typ = {PUB:(DE-HGF)16},
pubmed = {pmid:34871694},
UT = {WOS:000740193300016},
doi = {10.1016/j.scitotenv.2021.152141},
url = {https://juser.fz-juelich.de/record/907341},
}