000907439 001__ 907439
000907439 005__ 20240109115102.0
000907439 0247_ $$2doi$$a10.1038/s44160-022-00038-z
000907439 0247_ $$2Handle$$a2128/31095
000907439 0247_ $$2altmetric$$aaltmetric:124644004
000907439 0247_ $$2WOS$$aWOS:001126670400011
000907439 037__ $$aFZJ-2022-02037
000907439 041__ $$aEnglish
000907439 082__ $$a610
000907439 1001_ $$0P:(DE-HGF)0$$aGuo, Shasha$$b0
000907439 245__ $$aDirect growth of single-metal-atom chains
000907439 260__ $$aLondon$$bNature Publishing Group UK$$c2022
000907439 3367_ $$2DRIVER$$aarticle
000907439 3367_ $$2DataCite$$aOutput Types/Journal article
000907439 3367_ $$0PUB:(DE-HGF)16$$2PUB:(DE-HGF)$$aJournal Article$$bjournal$$mjournal$$s1651482161_16137
000907439 3367_ $$2BibTeX$$aARTICLE
000907439 3367_ $$2ORCID$$aJOURNAL_ARTICLE
000907439 3367_ $$00$$2EndNote$$aJournal Article
000907439 520__ $$aSingle-metal-atom chains (SMACs), as the smallest one-dimensional structure, have intriguing physical and chemical properties. Although several SMACs have been realized so far, their controllable fabrication remains challenging due to the need to arrange single atoms in an atomically precise manner. Here we develop a chemical vapour co-deposition method to construct a wafer-scale network of platinum SMACs in atom-thin films. The obtained atomic chains possess an average length of up to ~17 nm and a high density of over 10 wt%. Interestingly, as a consequence of the electronic delocalization of platinum atoms along the chain, this atomically coherent one-dimensional channel delivers a metallic behaviour, as revealed by electronic measurements, first-principles calculations and complex network modelling. Our strategy is potentially extendable to other transition metals such as cobalt, enriching the toolbox for manufacturing SMACs and paving the way for the fundamental study of one-dimensional systems and the development of devices comprising monoatomic chains.
000907439 536__ $$0G:(DE-HGF)POF4-5353$$a5353 - Understanding the Structural and Functional Behavior of Solid State Systems (POF4-535)$$cPOF4-535$$fPOF IV$$x0
000907439 536__ $$0G:(DE-HGF)POF4-5351$$a5351 - Platform for Correlative, In Situ and Operando Characterization (POF4-535)$$cPOF4-535$$fPOF IV$$x1
000907439 536__ $$0G:(GEPRIS)167917811$$aDFG project 167917811 - SFB 917: Resistiv schaltende Chalkogenide für zukünftige Elektronikanwendungen: Struktur, Kinetik und Bauelementskalierung "Nanoswitches" (167917811)$$c167917811$$x2
000907439 588__ $$aDataset connected to CrossRef, Journals: juser.fz-juelich.de
000907439 65027 $$0V:(DE-MLZ)SciArea-180$$2V:(DE-HGF)$$aMaterials Science$$x0
000907439 65027 $$0V:(DE-MLZ)SciArea-110$$2V:(DE-HGF)$$aChemistry$$x1
000907439 65027 $$0V:(DE-MLZ)SciArea-120$$2V:(DE-HGF)$$aCondensed Matter Physics$$x2
000907439 7001_ $$0P:(DE-HGF)0$$aFu, Jiecai$$b1
000907439 7001_ $$0P:(DE-HGF)0$$aZhang, Peikun$$b2
000907439 7001_ $$00000-0001-6383-3665$$aZhu, Chao$$b3
000907439 7001_ $$0P:(DE-HGF)0$$aYao, Heming$$b4
000907439 7001_ $$00000-0001-6752-5299$$aXu, Manzhang$$b5
000907439 7001_ $$0P:(DE-HGF)0$$aAn, Boxing$$b6
000907439 7001_ $$00000-0003-2411-7804$$aWang, Xingli$$b7
000907439 7001_ $$0P:(DE-HGF)0$$aTang, Bijun$$b8
000907439 7001_ $$0P:(DE-Juel1)190782$$aDeng, Yan$$b9
000907439 7001_ $$0P:(DE-HGF)0$$aSalim, Teddy$$b10
000907439 7001_ $$0P:(DE-Juel1)145710$$aDu, Hongchu$$b11
000907439 7001_ $$0P:(DE-Juel1)144121$$aDunin-Borkowski, Rafal$$b12$$ufzj
000907439 7001_ $$0P:(DE-HGF)0$$aXu, Mingquan$$b13
000907439 7001_ $$00000-0002-6803-1095$$aZhou, Wu$$b14
000907439 7001_ $$0P:(DE-HGF)0$$aTay, Beng Kang$$b15
000907439 7001_ $$0P:(DE-HGF)0$$aZhu, Chao$$b16
000907439 7001_ $$00000-0002-3227-0780$$aHe, Yanchao$$b17
000907439 7001_ $$0P:(DE-HGF)0$$aHofmann, Mario$$b18
000907439 7001_ $$0P:(DE-HGF)0$$aHsieh, Ya-Ping$$b19
000907439 7001_ $$0P:(DE-HGF)0$$aGuo, Wanlin$$b20
000907439 7001_ $$00000-0001-6833-5227$$aNg, Michael$$b21
000907439 7001_ $$0P:(DE-Juel1)130736$$aJia, Chun-Lin$$b22$$eCorresponding author
000907439 7001_ $$00000-0001-6406-0959$$aZhang, Zhuhua$$b23$$eCorresponding author
000907439 7001_ $$00000-0002-9347-930X$$aHe, Yongmin$$b24$$eCorresponding author
000907439 7001_ $$00000-0002-8825-7198$$aLiu, Zheng$$b25$$eCorresponding author
000907439 773__ $$0PERI:(DE-600)3105490-0$$a10.1038/s44160-022-00038-z$$gVol. 1, no. 3, p. 245 - 253$$n3$$p245 - 253$$tNature Synthesis$$v1$$x2731-0582$$y2022
000907439 8564_ $$uhttps://juser.fz-juelich.de/record/907439/files/s44160-022-00038-z-1.pdf
000907439 8564_ $$uhttps://juser.fz-juelich.de/record/907439/files/Direct%20growth.pdf$$yPublished on 2022-03-14. Available in OpenAccess from 2022-09-14.
000907439 909CO $$ooai:juser.fz-juelich.de:907439$$pdnbdelivery$$pdriver$$pVDB$$popen_access$$popenaire
000907439 9101_ $$0I:(DE-588b)5008462-8$$6P:(DE-Juel1)145710$$aForschungszentrum Jülich$$b11$$kFZJ
000907439 9101_ $$0I:(DE-588b)36225-6$$6P:(DE-Juel1)145710$$aRWTH Aachen$$b11$$kRWTH
000907439 9101_ $$0I:(DE-588b)5008462-8$$6P:(DE-Juel1)144121$$aForschungszentrum Jülich$$b12$$kFZJ
000907439 9101_ $$0I:(DE-588b)5008462-8$$6P:(DE-Juel1)130736$$aForschungszentrum Jülich$$b22$$kFZJ
000907439 9101_ $$0I:(DE-HGF)0$$60000-0001-6406-0959$$aExternal Institute$$b23$$kExtern
000907439 9101_ $$0I:(DE-HGF)0$$60000-0002-9347-930X$$aExternal Institute$$b24$$kExtern
000907439 9101_ $$0I:(DE-HGF)0$$60000-0002-8825-7198$$aExternal Institute$$b25$$kExtern
000907439 9131_ $$0G:(DE-HGF)POF4-535$$1G:(DE-HGF)POF4-530$$2G:(DE-HGF)POF4-500$$3G:(DE-HGF)POF4$$4G:(DE-HGF)POF$$9G:(DE-HGF)POF4-5353$$aDE-HGF$$bKey Technologies$$lMaterials Systems Engineering$$vMaterials Information Discovery$$x0
000907439 9131_ $$0G:(DE-HGF)POF4-535$$1G:(DE-HGF)POF4-530$$2G:(DE-HGF)POF4-500$$3G:(DE-HGF)POF4$$4G:(DE-HGF)POF$$9G:(DE-HGF)POF4-5351$$aDE-HGF$$bKey Technologies$$lMaterials Systems Engineering$$vMaterials Information Discovery$$x1
000907439 9141_ $$y2022
000907439 915__ $$0StatID:(DE-HGF)0530$$2StatID$$aEmbargoed OpenAccess
000907439 915__ $$0StatID:(DE-HGF)0300$$2StatID$$aDBCoverage$$bMedline$$d2022-11-30
000907439 920__ $$lyes
000907439 9201_ $$0I:(DE-Juel1)ER-C-2-20170209$$kER-C-2$$lMaterialwissenschaft u. Werkstofftechnik$$x0
000907439 9201_ $$0I:(DE-Juel1)ER-C-1-20170209$$kER-C-1$$lPhysik Nanoskaliger Systeme$$x1
000907439 980__ $$ajournal
000907439 980__ $$aVDB
000907439 980__ $$aUNRESTRICTED
000907439 980__ $$aI:(DE-Juel1)ER-C-2-20170209
000907439 980__ $$aI:(DE-Juel1)ER-C-1-20170209
000907439 9801_ $$aFullTexts