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@ARTICLE{Guo:907439,
author = {Guo, Shasha and Fu, Jiecai and Zhang, Peikun and Zhu, Chao
and Yao, Heming and Xu, Manzhang and An, Boxing and Wang,
Xingli and Tang, Bijun and Deng, Yan and Salim, Teddy and
Du, Hongchu and Dunin-Borkowski, Rafal and Xu, Mingquan and
Zhou, Wu and Tay, Beng Kang and Zhu, Chao and He, Yanchao
and Hofmann, Mario and Hsieh, Ya-Ping and Guo, Wanlin and
Ng, Michael and Jia, Chun-Lin and Zhang, Zhuhua and He,
Yongmin and Liu, Zheng},
title = {{D}irect growth of single-metal-atom chains},
journal = {Nature Synthesis},
volume = {1},
number = {3},
issn = {2731-0582},
address = {London},
publisher = {Nature Publishing Group UK},
reportid = {FZJ-2022-02037},
pages = {245 - 253},
year = {2022},
abstract = {Single-metal-atom chains (SMACs), as the smallest
one-dimensional structure, have intriguing physical and
chemical properties. Although several SMACs have been
realized so far, their controllable fabrication remains
challenging due to the need to arrange single atoms in an
atomically precise manner. Here we develop a chemical vapour
co-deposition method to construct a wafer-scale network of
platinum SMACs in atom-thin films. The obtained atomic
chains possess an average length of up to ~17 nm and a
high density of over $10 wt\%.$ Interestingly, as a
consequence of the electronic delocalization of platinum
atoms along the chain, this atomically coherent
one-dimensional channel delivers a metallic behaviour, as
revealed by electronic measurements, first-principles
calculations and complex network modelling. Our strategy is
potentially extendable to other transition metals such as
cobalt, enriching the toolbox for manufacturing SMACs and
paving the way for the fundamental study of one-dimensional
systems and the development of devices comprising monoatomic
chains.},
cin = {ER-C-2 / ER-C-1},
ddc = {610},
cid = {I:(DE-Juel1)ER-C-2-20170209 / I:(DE-Juel1)ER-C-1-20170209},
pnm = {5353 - Understanding the Structural and Functional Behavior
of Solid State Systems (POF4-535) / 5351 - Platform for
Correlative, In Situ and Operando Characterization
(POF4-535) / DFG project 167917811 - SFB 917: Resistiv
schaltende Chalkogenide für zukünftige
Elektronikanwendungen: Struktur, Kinetik und
Bauelementskalierung "Nanoswitches" (167917811)},
pid = {G:(DE-HGF)POF4-5353 / G:(DE-HGF)POF4-5351 /
G:(GEPRIS)167917811},
typ = {PUB:(DE-HGF)16},
UT = {WOS:001126670400011},
doi = {10.1038/s44160-022-00038-z},
url = {https://juser.fz-juelich.de/record/907439},
}