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@ARTICLE{He:907453,
      author       = {He, Yongmin and Liu, Liren and Zhu, Chao and Guo, Shasha
                      and Golani, Prafful and Koo, Bonhyeong and Tang, Pengyi and
                      Zhao, Zhiqiang and Xu, Manzhang and Zhu, Chao and Yu, Peng
                      and Zhou, Xin and Gao, Caitian and Wang, Xuewen and Shi,
                      Zude and Zheng, Lu and Yang, Jiefu and Shin, Byungha and
                      Arbiol, Jordi and Duan, Huigao and Du, Yonghua and Heggen,
                      Marc and Dunin-Borkowski, Rafal E. and Guo, Wanlin and Wang,
                      Qin and Zhang, Zhuhua and Liu, Zheng},
      title        = {{A}morphizing noble metal chalcogenide catalysts at the
                      single-layer limit towards hydrogen production},
      journal      = {Nature catalysis},
      volume       = {5},
      number       = {3},
      issn         = {2520-1158},
      address      = {[London]},
      publisher    = {Macmillan Publishers Limited, part of Springer Nature},
      reportid     = {FZJ-2022-02045},
      pages        = {212 - 221},
      year         = {2022},
      abstract     = {Rational design of noble metal catalysts with the potential
                      to leverage efficiency is vital for industrial applications.
                      Such an ultimate atom-utilization efficiency can be achieved
                      when all noble metal atoms exclusively contribute to
                      catalysis. Here, we demonstrate the fabrication of a
                      wafer-size amorphous PtSex film on a SiO2 substate via a
                      low-temperature amorphization strategy, which offers
                      single-atom-layer Pt catalysts with high atom-utilization
                      efficiency $(~26 wt\%).$ This amorphous PtSex
                      (1.2 < x < 1.3) behaves as a fully activated
                      surface, accessible to catalytic reactions, and features a
                      nearly $100\%$ current density relative to a pure Pt surface
                      and reliable production of sustained high-flux hydrogen over
                      a 2 inch wafer as a proof-of-concept. Furthermore, an
                      electrolyser is demonstrated to generate a high current
                      density of 1,000 mA cm−2. Such an amorphization
                      strategy is potentially extendable to other noble metals,
                      including the Pd, Ir, Os, Rh and Ru elements, demonstrating
                      the universality of single-atom-layer catalysts.},
      cin          = {ER-C-1},
      ddc          = {540},
      cid          = {I:(DE-Juel1)ER-C-1-20170209},
      pnm          = {5351 - Platform for Correlative, In Situ and Operando
                      Characterization (POF4-535) / ESTEEM3 - Enabling Science and
                      Technology through European Electron Microscopy (823717)},
      pid          = {G:(DE-HGF)POF4-5351 / G:(EU-Grant)823717},
      typ          = {PUB:(DE-HGF)16},
      UT           = {WOS:000766418700001},
      doi          = {10.1038/s41929-022-00753-y},
      url          = {https://juser.fz-juelich.de/record/907453},
}