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@ARTICLE{Chiou:907665,
author = {Chiou, Min-Huei and Borzutzki, Kristina and Thienenkamp,
Johannes Helmut and Mohrhardt, Marvin and Liu, Kun Ling and
Mereacre, Valeriu and Binder, Joachim R. and Ehrenberg,
Helmut and Winter, Martin and Brunklaus, Gunther},
title = {{D}urable fast-charging lithium metal batteries designed
with cross-linked polymer electrolytes and niobate-coated
cathode},
journal = {Journal of power sources},
volume = {538},
issn = {0378-7753},
address = {New York, NY [u.a.]},
publisher = {Elsevier},
reportid = {FZJ-2022-02142},
pages = {231528 -},
year = {2022},
abstract = {A durable lithium metal polymer battery with extended
cycle-life is designed by exploiting cross-linked
poly(trimethylene carbonate) (PTMC) electrolytes and
LiNi0.6Mn0.2Co0.2O2 (NMC622) with well-defined
protectivecoating (0.5 $wt\%$ of LiNbO3 on the surface
layer, <5 nm thickness). The presented materials
demonstratefeasibility of faster cycling at rates of 1C and
2C at temperatures of 40 and 60 ◦C, exhibiting prominent
capacityretention of $91\%$ and $80\%$ SOH (state of health)
after 500 cycles. At higher cross-linking densities, the
introducedquasi-solid polymer electrolytes afford good
cycling performance and sufficient suppression of high
surface arealithium depositions as well as improved ability
of solvent entrapment, hence reflecting a considerable
stepforward towards achieving all solid-state polymer-based
cells.},
cin = {IEK-12},
ddc = {620},
cid = {I:(DE-Juel1)IEK-12-20141217},
pnm = {1221 - Fundamentals and Materials (POF4-122)},
pid = {G:(DE-HGF)POF4-1221},
typ = {PUB:(DE-HGF)16},
UT = {WOS:000798957800003},
doi = {10.1016/j.jpowsour.2022.231528},
url = {https://juser.fz-juelich.de/record/907665},
}