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@ARTICLE{Guasco:907713,
author = {Guasco, L. and Khaydukov, Yu. N. and Pütter, S. and Silvi,
L. and Paulin, M. A. and Keller, T. and Keimer, B.},
title = {{R}esonant neutron reflectometry for hydrogen detection},
journal = {Nature Communications},
volume = {13},
number = {1},
issn = {2041-1723},
address = {[London]},
publisher = {Nature Publishing Group UK},
reportid = {FZJ-2022-02176},
pages = {1486},
year = {2022},
abstract = {The detection and quantification of hydrogen is becoming
increasingly important in research on electronic materials
and devices, following the identification of the hydrogen
content as a potent control parameter for the electronic
properties. However, establishing quantitative correlations
between the hydrogen content and the physical properties of
solids remains a formidable challenge. Here we report
neutron reflectometry experiments on 50 nm thick niobium
films during hydrogen loading, and show that the
momentum-space position of a prominent waveguide resonance
allows tracking of the absolute hydrogen content with an
accuracy of about one atomic percent on a timescale of less
than a minute. Resonance-enhanced neutron reflectometry thus
allows fast, direct, and non-destructive measurements of the
hydrogen concentration in thin-film structures, with
sensitivity high enough for real-time in-situ studies.},
cin = {JCNS-4 / MLZ},
ddc = {500},
cid = {I:(DE-Juel1)JCNS-4-20201012 / I:(DE-588b)4597118-3},
pnm = {6G4 - Jülich Centre for Neutron Research (JCNS) (FZJ)
(POF4-6G4) / 622 - Detector Technologies and Systems
(POF4-622)},
pid = {G:(DE-HGF)POF4-6G4 / G:(DE-HGF)POF4-622},
experiment = {EXP:(DE-MLZ)MBE-MLZ-20151210 / EXP:(DE-MLZ)N-REX-20140101},
typ = {PUB:(DE-HGF)16},
pubmed = {35304444},
UT = {WOS:000770716000011},
doi = {10.1038/s41467-022-29092-z},
url = {https://juser.fz-juelich.de/record/907713},
}