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000907823 1001_ $$0P:(DE-Juel1)169518$$aJovanovic, Sven$$b0
000907823 245__ $$aPolysiloxane‐Based Single‐Ion Conducting Polymer Blend Electrolyte Comprising Small‐Molecule Organic Carbonates for High‐Energy and High‐Power Lithium‐Metal Batteries
000907823 260__ $$aWeinheim$$bWiley-VCH$$c2022
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000907823 520__ $$aSingle-ion conducting polymer electrolytes are considered particularly attractive for realizing high-performance solid-state lithium-metal batteries. Herein, a polysiloxane-based single-ion conductor (PSiO) is investigated. The synthesis is performed via a simple thiol-ene reaction, yielding flexible and self-standing polymer electrolyte membranes (PSiOM) when blended with poly(vinylidene fluoride-co-hexafluoropropylene) (PVdF-HFP). When incorporating 57 wt% of organic carbonates, these polymer membranes provide a Li+ conductivity of >0.4 mS cm−1 at 20 °C and a wide electrochemical stability window of more than 4.8 V. This excellent electrochemical stability allows for the highly reversible cycling of symmetric Li||Li cells as well as high-energy Li||LiNi0.6Mn0.2Co0.2O2 (NMC622) and Li||LiNi0.8Mn0.1Co0.1O2 (NMC811) cells for several hundred cycles at relatively high discharge and charge rates. Remarkably, Li||NMC811 cells with high mass loading cathodes provide more than 76% capacity retention at a high current density of 1.44 mA cm−2, thus rendering this polymer electrolyte suitable for high-performance battery applications.
000907823 536__ $$0G:(DE-HGF)POF4-1223$$a1223 - Batteries in Application (POF4-122)$$cPOF4-122$$fPOF IV$$x0
000907823 536__ $$0G:(BMBF)13XP0176B$$aFestBatt-Charakterisierung - Methodenplattform 'Charakterisierung' im Rahmen des Kompetenzclusters für Festkörperbatterien (13XP0176B)$$c13XP0176B$$x1
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000907823 7001_ $$0P:(DE-HGF)0$$aLiang, Hai-Peng$$b1$$eCorresponding author
000907823 7001_ $$0P:(DE-HGF)0$$aZarrabeitia, Maider$$b2
000907823 7001_ $$0P:(DE-Juel1)180579$$aChen, Zhen$$b3
000907823 7001_ $$0P:(DE-Juel1)129503$$aMerz, Steffen$$b4
000907823 7001_ $$0P:(DE-Juel1)162401$$aGranwehr, Josef$$b5
000907823 7001_ $$00000-0002-6606-5304$$aPasserini, Stefano$$b6
000907823 7001_ $$0P:(DE-HGF)0$$aBresser, Dominic$$b7$$eCorresponding author
000907823 773__ $$0PERI:(DE-600)2594556-7$$a10.1002/aenm.202200013$$gVol. 12, no. 16, p. 2200013 -$$n16$$p2200013 -$$tAdvanced energy materials$$v12$$x1614-6832$$y2022
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