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@ARTICLE{Jovanovic:907823,
      author       = {Jovanovic, Sven and Liang, Hai-Peng and Zarrabeitia, Maider
                      and Chen, Zhen and Merz, Steffen and Granwehr, Josef and
                      Passerini, Stefano and Bresser, Dominic},
      title        = {{P}olysiloxane‐{B}ased {S}ingle‐{I}on {C}onducting
                      {P}olymer {B}lend {E}lectrolyte {C}omprising
                      {S}mall‐{M}olecule {O}rganic {C}arbonates for
                      {H}igh‐{E}nergy and {H}igh‐{P}ower {L}ithium‐{M}etal
                      {B}atteries},
      journal      = {Advanced energy materials},
      volume       = {12},
      number       = {16},
      issn         = {1614-6832},
      address      = {Weinheim},
      publisher    = {Wiley-VCH},
      reportid     = {FZJ-2022-02234},
      pages        = {2200013 -},
      year         = {2022},
      abstract     = {Single-ion conducting polymer electrolytes are considered
                      particularly attractive for realizing high-performance
                      solid-state lithium-metal batteries. Herein, a
                      polysiloxane-based single-ion conductor (PSiO) is
                      investigated. The synthesis is performed via a simple
                      thiol-ene reaction, yielding flexible and self-standing
                      polymer electrolyte membranes (PSiOM) when blended with
                      poly(vinylidene fluoride-co-hexafluoropropylene) (PVdF-HFP).
                      When incorporating 57 $wt\%$ of organic carbonates, these
                      polymer membranes provide a Li+ conductivity of >0.4 mS
                      cm−1 at 20 °C and a wide electrochemical stability window
                      of more than 4.8 V. This excellent electrochemical stability
                      allows for the highly reversible cycling of symmetric Li||Li
                      cells as well as high-energy Li||LiNi0.6Mn0.2Co0.2O2
                      (NMC622) and Li||LiNi0.8Mn0.1Co0.1O2 (NMC811) cells for
                      several hundred cycles at relatively high discharge and
                      charge rates. Remarkably, Li||NMC811 cells with high mass
                      loading cathodes provide more than $76\%$ capacity retention
                      at a high current density of 1.44 mA cm−2, thus rendering
                      this polymer electrolyte suitable for high-performance
                      battery applications.},
      cin          = {IEK-9},
      ddc          = {050},
      cid          = {I:(DE-Juel1)IEK-9-20110218},
      pnm          = {1223 - Batteries in Application (POF4-122) /
                      FestBatt-Charakterisierung - Methodenplattform
                      'Charakterisierung' im Rahmen des Kompetenzclusters für
                      Festkörperbatterien (13XP0176B)},
      pid          = {G:(DE-HGF)POF4-1223 / G:(BMBF)13XP0176B},
      typ          = {PUB:(DE-HGF)16},
      UT           = {WOS:000767680200001},
      doi          = {10.1002/aenm.202200013},
      url          = {https://juser.fz-juelich.de/record/907823},
}