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| 024 | 7 | _ | |a 10.1002/aenm.202200013 |2 doi |
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| 100 | 1 | _ | |a Jovanovic, Sven |0 P:(DE-Juel1)169518 |b 0 |
| 245 | _ | _ | |a Polysiloxane‐Based Single‐Ion Conducting Polymer Blend Electrolyte Comprising Small‐Molecule Organic Carbonates for High‐Energy and High‐Power Lithium‐Metal Batteries |
| 260 | _ | _ | |a Weinheim |c 2022 |b Wiley-VCH |
| 336 | 7 | _ | |a article |2 DRIVER |
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| 520 | _ | _ | |a Single-ion conducting polymer electrolytes are considered particularly attractive for realizing high-performance solid-state lithium-metal batteries. Herein, a polysiloxane-based single-ion conductor (PSiO) is investigated. The synthesis is performed via a simple thiol-ene reaction, yielding flexible and self-standing polymer electrolyte membranes (PSiOM) when blended with poly(vinylidene fluoride-co-hexafluoropropylene) (PVdF-HFP). When incorporating 57 wt% of organic carbonates, these polymer membranes provide a Li+ conductivity of >0.4 mS cm−1 at 20 °C and a wide electrochemical stability window of more than 4.8 V. This excellent electrochemical stability allows for the highly reversible cycling of symmetric Li||Li cells as well as high-energy Li||LiNi0.6Mn0.2Co0.2O2 (NMC622) and Li||LiNi0.8Mn0.1Co0.1O2 (NMC811) cells for several hundred cycles at relatively high discharge and charge rates. Remarkably, Li||NMC811 cells with high mass loading cathodes provide more than 76% capacity retention at a high current density of 1.44 mA cm−2, thus rendering this polymer electrolyte suitable for high-performance battery applications. |
| 536 | _ | _ | |a 1223 - Batteries in Application (POF4-122) |0 G:(DE-HGF)POF4-1223 |c POF4-122 |f POF IV |x 0 |
| 536 | _ | _ | |a FestBatt-Charakterisierung - Methodenplattform 'Charakterisierung' im Rahmen des Kompetenzclusters für Festkörperbatterien (13XP0176B) |0 G:(BMBF)13XP0176B |c 13XP0176B |x 1 |
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| 700 | 1 | _ | |a Liang, Hai-Peng |0 P:(DE-HGF)0 |b 1 |e Corresponding author |
| 700 | 1 | _ | |a Zarrabeitia, Maider |0 P:(DE-HGF)0 |b 2 |
| 700 | 1 | _ | |a Chen, Zhen |0 P:(DE-Juel1)180579 |b 3 |
| 700 | 1 | _ | |a Merz, Steffen |0 P:(DE-Juel1)129503 |b 4 |
| 700 | 1 | _ | |a Granwehr, Josef |0 P:(DE-Juel1)162401 |b 5 |
| 700 | 1 | _ | |a Passerini, Stefano |0 0000-0002-6606-5304 |b 6 |
| 700 | 1 | _ | |a Bresser, Dominic |0 P:(DE-HGF)0 |b 7 |e Corresponding author |
| 773 | _ | _ | |a 10.1002/aenm.202200013 |g Vol. 12, no. 16, p. 2200013 - |0 PERI:(DE-600)2594556-7 |n 16 |p 2200013 - |t Advanced energy materials |v 12 |y 2022 |x 1614-6832 |
| 856 | 4 | _ | |u https://juser.fz-juelich.de/record/907823/files/Advanced%20Energy%20Materials%20-%202022%20-%20Liang%20-%20Polysiloxane%E2%80%90Based%20Single%E2%80%90Ion%20Conducting%20Polymer%20Blend%20Electrolyte%20Comprising.pdf |y OpenAccess |
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