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@ARTICLE{Wrogemann:907890,
      author       = {Wrogemann, Jens Matthies and Haneke, Lukas and Ramireddy,
                      Thrinathreddy and Frerichs, Joop Enno and Sultana, Irin and
                      Chen, Ying Ian and Brink, Frank and Hansen, Michael Ryan and
                      Winter, Martin and Glushenkov, Alexey M. and Placke, Tobias},
      title        = {{A}dvanced {D}ual‐{I}on {B}atteries with
                      {H}igh‐{C}apacity {N}egative {E}lectrodes {I}ncorporating
                      {B}lack {P}hosphorus},
      journal      = {Advanced science},
      volume       = {9},
      number       = {20},
      issn         = {2198-3844},
      address      = {Weinheim},
      publisher    = {Wiley-VCH},
      reportid     = {FZJ-2022-02269},
      pages        = {2201116 -},
      year         = {2022},
      abstract     = {Dual-graphite batteries (DGBs), being an
                      all-graphite-electrode variation of dual-ion batteries
                      (DIBs), have attracted great attention in recent years as a
                      possible low-cost technology for stationary energy storage
                      due to the utilization of inexpensive graphite as a positive
                      electrode (cathode) material. However, DGBs suffer from a
                      low specific energy limited by the capacity of both
                      electrode materials. In this work, a composite of black
                      phosphorus with carbon (BP-C) is introduced as negative
                      electrode (anode) material for DIB full-cells for the first
                      time. The electrochemical behavior of the graphite || BP-C
                      DIB cells is then discussed in the context of DGBs and DIBs
                      using alloying anodes. Mechanistic studies confirm the
                      staging behavior for anion storage in the graphite positive
                      electrode and the formation of lithiated phosphorus alloys
                      in the negative electrode. BP-C containing full-cells
                      demonstrate promising electrochemical performance with
                      specific energies of up to 319 Wh kg–1 (related to masses
                      of both electrode active materials) or 155 Wh kg–1
                      (related to masses of electrode active materials and active
                      salt), and high Coulombic efficiency. This work provides
                      highly relevant insights for the development of advanced
                      high-energy and safe DIBs incorporating BP-C and other
                      high-capacity alloying materials in their anodes.},
      cin          = {IEK-12},
      ddc          = {624},
      cid          = {I:(DE-Juel1)IEK-12-20141217},
      pnm          = {1221 - Fundamentals and Materials (POF4-122)},
      pid          = {G:(DE-HGF)POF4-1221},
      typ          = {PUB:(DE-HGF)16},
      pubmed       = {35474449},
      UT           = {WOS:000787737100001},
      doi          = {10.1002/advs.202201116},
      url          = {https://juser.fz-juelich.de/record/907890},
}