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@ARTICLE{Reber:907896,
      author       = {Reber, David and Borodin, Oleg and Becker, Maximilian and
                      Rentsch, Daniel and Thienenkamp, Johannes Helmut and Grissa,
                      Rabeb and Zhao, Wengao and Aribia, Abdessalem and Brunklaus,
                      Gunther and Battaglia, Corsin and Kühnel, Ruben-Simon},
      title        = {{W}ater/{I}onic {L}iquid/{S}uccinonitrile {H}ybrid
                      {E}lectrolytes for {A}queous {B}atteries},
      journal      = {Advanced functional materials},
      volume       = {32},
      number       = {20},
      issn         = {1057-9257},
      address      = {Weinheim},
      publisher    = {Wiley-VCH},
      reportid     = {FZJ-2022-02274},
      pages        = {2112138},
      year         = {2022},
      note         = {Funding: Swiss National Science Foundation
                      $206021_150638/1$},
      abstract     = {The water-in-salt concept has significantly improved the
                      electrochemical stability of aqueous electrolytes, and the
                      hybridization with organic solvents or ionic liquids has
                      further enhanced their reductive stability, enabling cell
                      chemistries with up to 150 Wh kg−1 of active material.
                      Here, a large design space is opened by introducing
                      succinonitrile as a cosolvent in water/ionic
                      liquid/succinonitrile hybrid electrolytes (WISHEs). By means
                      of succinonitrile addition, the solubility limits can be
                      fully circumvented, and the properties of the electrolytes
                      can be optimized for various metrics such as highest
                      electrochemical stability, maximum conductivity, or lowest
                      cost. While excessive nitrile fractions render the mixtures
                      flammable, careful selection of component ratios yields
                      highly performant, nonflammable electrolytes that enable
                      stable cycling of Li4Ti5O12–LiNi0.8Mn0.1Co0.1O2 full cells
                      over a wide temperature range with strong rate performance,
                      facilitated by the fast conformational dynamics of
                      succinonitrile. The WISHEs allow stable cycling with a
                      maximum energy density of ≈140 Wh kg−1 of active
                      material, Coulombic efficiencies of close to $99.5\%$ at 1C,
                      and a capacity retention of $53\%$ at 10C relative to 1C.},
      cin          = {IEK-12},
      ddc          = {530},
      cid          = {I:(DE-Juel1)IEK-12-20141217},
      pnm          = {1221 - Fundamentals and Materials (POF4-122)},
      pid          = {G:(DE-HGF)POF4-1221},
      typ          = {PUB:(DE-HGF)16},
      UT           = {WOS:000761531600001},
      doi          = {10.1002/adfm.202112138},
      url          = {https://juser.fz-juelich.de/record/907896},
}