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| Hauptseite > Workflowsammlungen > Publikationsgebühren > Characterization of Y and Mn co-substituted BaZrO3 ceramics: Material properties as a function of the substituent concentration > print |
| Hauptseite > Workflowsammlungen > Publikationsgebühren > Characterization of Y and Mn co-substituted BaZrO3 ceramics: Material properties as a function of the substituent concentration > print |
| 001 | 908321 | ||
| 005 | 20240711085621.0 | ||
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| 100 | 1 | _ | |a Balaguer, Maria |0 P:(DE-Juel1)161336 |b 0 |e Corresponding author |
| 245 | _ | _ | |a Characterization of Y and Mn co-substituted BaZrO3 ceramics: Material properties as a function of the substituent concentration |
| 260 | _ | _ | |a Amsterdam [u.a.] |c 2022 |b Elsevier Science |
| 336 | 7 | _ | |a article |2 DRIVER |
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| 520 | _ | _ | |a Innovations in materials science are the key element for solving technological challenges. Various energy and environmental applications require designing materials with tailored compositions, microstructures and specific target-oriented performance. Y and Mn co-substituted BaZrO3, e.g. BaZr0.85Y0.15Mn0.05O3-δ, has previously attracted attention as a membrane material for H2 separation from gas mixtures due to its mixed proton-electron conductivity leading to appreciable levels of H2-flux at elevated temperatures and its good thermo-chemical stability under reducing environments. In the present work, we developed ceramic materials within the BaZr0.8Y0.2-xMnxO3-δ series, where x = 0.02–0.15. The study of their functional properties in dependence of the Y-to-Mn ratio disclosed that thermal expansion and hydration decrease by increasing the Mn content as well as the total electrical conductivity. In addition to that, XPS analysis and near edge X-ray absorption fine structure spectra (NEXAFS) in the vicinity of O K-edge and Mn L2,3-edges indicated that the Mn atoms oxidation state in the surface and in the bulk range from Mn2+ to Mn4+ depending on the ambient conditions that can be encountered in MPEC electrodes, which it is suggested to be related with a hydration mechanism mediated by Mn oxidation and subsequent proton attachment to oxygen neighbors, similar to LSM. |
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| 700 | 1 | _ | |a Sohn, Yoo Jung |0 P:(DE-Juel1)159368 |b 1 |u fzj |
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| 773 | _ | _ | |a 10.1016/j.ssi.2022.115959 |g Vol. 382, p. 115959 - |0 PERI:(DE-600)1500750-9 |p 115959 - |t Solid state ionics |v 382 |y 2022 |x 0167-2738 |
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