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@ARTICLE{Chen:908636,
      author       = {Chen, Yi-Hsuan and Hsieh, Yi-Chen and Liu, Kun Ling and
                      Wichmann, Lennart and Thienenkamp, Johannes Helmut and
                      Choudhary, Aditya and Bedrov, Dmitry and Winter, Martin and
                      Brunklaus, Gunther},
      title        = {{G}reen {P}olymer {E}lectrolytes {B}ased on
                      {P}olycaprolactones for {S}olid‐{S}tate {H}igh‐{V}oltage
                      {L}ithium {M}etal {B}atteries},
      journal      = {Macromolecular rapid communications},
      volume       = {43},
      number       = {20},
      issn         = {0173-2803},
      address      = {Weinheim},
      publisher    = {Wiley-VCH},
      reportid     = {FZJ-2022-02735},
      pages        = {2200335},
      year         = {2022},
      note         = {Army Research Laboratory. Grant Number: W911NF-12-2-0023},
      abstract     = {Solid polymer electrolytes (SPEs) have attracted
                      considerable attention forhigh energy solid-state lithium
                      metal batteries (LMBs). In this work,
                      potentiallyecofriendly, solid-state poly(𝝐-caprolactone)
                      (PCL)-based star polymerelectrolytes with cross-linked
                      structures (xBt-PCL) are introduced that robustlycycle
                      against LiNi0.6Mn0.2Co0.2O2(NMC622) composite cathodes,
                      affordinglong-term stability even at higher current
                      densities. Their superior featuresallow for sufficient
                      suppression of dendritic lithium deposits, as monitored
                      by7Li solid-state NMR. Advantageous electrolyte|electrode
                      interfacial propertiesderived from cathode impregnation with
                      1.5 $wt\%$ PCL enable decent cellperformance until up to 500
                      cycles at rates of 1C (60°C), illustrating the
                      highpotential of PCL-based SPEs for application in
                      high-voltage LMBs.},
      cin          = {IEK-12},
      ddc          = {540},
      cid          = {I:(DE-Juel1)IEK-12-20141217},
      pnm          = {1223 - Batteries in Application (POF4-122) /
                      FestBatt-Polymere - Materialplattform 'Polymere' im Rahmen
                      des Kompetenzclusters für Festkörperbatterien (13XP0175A)
                      / LiBEST2 - Lithium-Batterie-Konzepte mit hoher
                      Energiedichte, Leistung und Sicherheit (13XP0304A) / LiSi -
                      Lithium-Solid-Electrolyte Interfaces (13XP0224A)},
      pid          = {G:(DE-HGF)POF4-1223 / G:(BMBF)13XP0175A / G:(BMBF)13XP0304A
                      / G:(BMBF)13XP0224A},
      typ          = {PUB:(DE-HGF)16},
      pubmed       = {35726135},
      UT           = {WOS:000819197500001},
      doi          = {10.1002/marc.202200335},
      url          = {https://juser.fz-juelich.de/record/908636},
}