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| 001 | 908636 | ||
| 005 | 20240712113115.0 | ||
| 024 | 7 | _ | |a 10.1002/marc.202200335 |2 doi |
| 024 | 7 | _ | |a 0173-2803 |2 ISSN |
| 024 | 7 | _ | |a 1022-1336 |2 ISSN |
| 024 | 7 | _ | |a 1521-3927 |2 ISSN |
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| 037 | _ | _ | |a FZJ-2022-02735 |
| 041 | _ | _ | |a English |
| 082 | _ | _ | |a 540 |
| 100 | 1 | _ | |a Chen, Yi-Hsuan |0 P:(DE-Juel1)178791 |b 0 |e First author |
| 245 | _ | _ | |a Green Polymer Electrolytes Based on Polycaprolactones for Solid‐State High‐Voltage Lithium Metal Batteries |
| 260 | _ | _ | |a Weinheim |c 2022 |b Wiley-VCH |
| 336 | 7 | _ | |a article |2 DRIVER |
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| 336 | 7 | _ | |a Journal Article |b journal |m journal |0 PUB:(DE-HGF)16 |s 1667570543_3685 |2 PUB:(DE-HGF) |
| 336 | 7 | _ | |a ARTICLE |2 BibTeX |
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| 500 | _ | _ | |a Army Research Laboratory. Grant Number: W911NF-12-2-0023 |
| 520 | _ | _ | |a Solid polymer electrolytes (SPEs) have attracted considerable attention forhigh energy solid-state lithium metal batteries (LMBs). In this work, potentiallyecofriendly, solid-state poly(𝝐-caprolactone) (PCL)-based star polymerelectrolytes with cross-linked structures (xBt-PCL) are introduced that robustlycycle against LiNi0.6Mn0.2Co0.2O2(NMC622) composite cathodes, affordinglong-term stability even at higher current densities. Their superior featuresallow for sufficient suppression of dendritic lithium deposits, as monitored by7Li solid-state NMR. Advantageous electrolyte|electrode interfacial propertiesderived from cathode impregnation with 1.5 wt% PCL enable decent cellperformance until up to 500 cycles at rates of 1C (60°C), illustrating the highpotential of PCL-based SPEs for application in high-voltage LMBs. |
| 536 | _ | _ | |a 1223 - Batteries in Application (POF4-122) |0 G:(DE-HGF)POF4-1223 |c POF4-122 |f POF IV |x 0 |
| 536 | _ | _ | |a FestBatt-Polymere - Materialplattform 'Polymere' im Rahmen des Kompetenzclusters für Festkörperbatterien (13XP0175A) |0 G:(BMBF)13XP0175A |c 13XP0175A |x 1 |
| 536 | _ | _ | |a LiBEST2 - Lithium-Batterie-Konzepte mit hoher Energiedichte, Leistung und Sicherheit (13XP0304A) |0 G:(BMBF)13XP0304A |c 13XP0304A |x 2 |
| 536 | _ | _ | |a LiSi - Lithium-Solid-Electrolyte Interfaces (13XP0224A) |0 G:(BMBF)13XP0224A |c 13XP0224A |x 3 |
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| 700 | 1 | _ | |a Hsieh, Yi-Chen |0 P:(DE-Juel1)174519 |b 1 |u fzj |
| 700 | 1 | _ | |a Liu, Kun Ling |0 P:(DE-Juel1)178047 |b 2 |u fzj |
| 700 | 1 | _ | |a Wichmann, Lennart |0 P:(DE-Juel1)187473 |b 3 |u fzj |
| 700 | 1 | _ | |a Thienenkamp, Johannes Helmut |0 P:(DE-Juel1)179050 |b 4 |u fzj |
| 700 | 1 | _ | |a Choudhary, Aditya |0 P:(DE-HGF)0 |b 5 |
| 700 | 1 | _ | |a Bedrov, Dmitry |0 P:(DE-HGF)0 |b 6 |
| 700 | 1 | _ | |a Winter, Martin |0 P:(DE-Juel1)166130 |b 7 |u fzj |
| 700 | 1 | _ | |a Brunklaus, Gunther |0 P:(DE-Juel1)172047 |b 8 |e Corresponding author |
| 773 | _ | _ | |a 10.1002/marc.202200335 |g p. 2200335 - |0 PERI:(DE-600)1475027-2 |n 20 |p 2200335 |t Macromolecular rapid communications |v 43 |y 2022 |x 0173-2803 |
| 856 | 4 | _ | |y OpenAccess |u https://juser.fz-juelich.de/record/908636/files/Green%20Polymer%20Electrolytes%20Based%20on%20Polycaprolactones%20for%20Solid%E2%80%90State%20High%E2%80%90Voltage%20Lithium%20Metal%20Batteries.pdf |
| 856 | 4 | _ | |y OpenAccess |u https://juser.fz-juelich.de/record/908636/files/Macromolecular%20Rapid%20Communications%20-%202022%20-%20Chen%20-%20Green%20Polymer%20Electrolytes%20Based%20on%20Polycaprolactones%20for%20Solid%E2%80%90State.pdf |
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