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000909075 1001_ $$0P:(DE-HGF)0$$aOverstreet, Cale$$b0
000909075 245__ $$aStructural stability of REE-PO4 (REE = Sm,Tb) under swift heavy ion irradiation
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000909075 520__ $$aRare earth element (REE) phosphates are an attractive host matrix for long-lived radionuclides from nuclear waste because of the radiation tolerance exhibited by naturally occurring REE phosphate specimens. Here we show that SmPO4 (monazite structure) and TbPO4 (xenotime structure) exhibit a similar amorphization response to swift heavy ion irradiation despite different starting structures. SmPO4 and TbPO4 were irradiated with 1.1 GeV Au ions and analyzed using synchrotron-based X-ray diffraction (XRD), Raman spectroscopy, and transmission electron microscopy (TEM). The radiation response of the phosphates was evaluated by extracting the amorphous fraction at each irradiation fluence, and a single-impact model was used to determine the amorphous cross section and track diameter. Amorphization within individual ion tracks was confirmed using head-on TEM imaging, and the amorphous track size agreed with the value deduced by XRD analysis. Raman measurements were performed to qualitatively confirm the ion-induced crystalline-to-amorphous transformation which proceeds similarly for both phosphates.
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000909075 7001_ $$0P:(DE-HGF)0$$aCooper, Jacob$$b1
000909075 7001_ $$0P:(DE-HGF)0$$aO'Quinn, Eric$$b2
000909075 7001_ $$0P:(DE-HGF)0$$aCureton, William$$b3
000909075 7001_ $$0P:(DE-HGF)0$$aPalomares, Raul$$b4
000909075 7001_ $$0P:(DE-HGF)0$$aLeys, Julia$$b5
000909075 7001_ $$0P:(DE-Juel1)156511$$aDeissmann, Guido$$b6
000909075 7001_ $$0P:(DE-Juel1)130389$$aNeumeier, Stefan$$b7
000909075 7001_ $$0P:(DE-HGF)0$$aChen, Chien-Hung$$b8
000909075 7001_ $$0P:(DE-HGF)0$$aLang, Maik$$b9$$eCorresponding author
000909075 773__ $$0PERI:(DE-600)1466524-4$$a10.1016/j.nimb.2022.07.014$$gVol. 527, p. 34 - 39$$p34 - 39$$tNuclear instruments & methods in physics research / B$$v527$$x0168-583X$$y2022
000909075 8564_ $$uhttps://juser.fz-juelich.de/record/909075/files/Overstreet%20NIMB%202022.pdf$$yPublished on 2022-08-06. Available in OpenAccess from 2024-08-06.
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