| Home > Publications database > Structural stability of REE-PO4 (REE = Sm,Tb) under swift heavy ion irradiation > print |
| 001 | 909075 | ||
| 005 | 20240708133959.0 | ||
| 024 | 7 | _ | |a 10.1016/j.nimb.2022.07.014 |2 doi |
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| 100 | 1 | _ | |a Overstreet, Cale |0 P:(DE-HGF)0 |b 0 |
| 245 | _ | _ | |a Structural stability of REE-PO4 (REE = Sm,Tb) under swift heavy ion irradiation |
| 260 | _ | _ | |a Amsterdam [u.a.] |c 2022 |b Elsevier |
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| 520 | _ | _ | |a Rare earth element (REE) phosphates are an attractive host matrix for long-lived radionuclides from nuclear waste because of the radiation tolerance exhibited by naturally occurring REE phosphate specimens. Here we show that SmPO4 (monazite structure) and TbPO4 (xenotime structure) exhibit a similar amorphization response to swift heavy ion irradiation despite different starting structures. SmPO4 and TbPO4 were irradiated with 1.1 GeV Au ions and analyzed using synchrotron-based X-ray diffraction (XRD), Raman spectroscopy, and transmission electron microscopy (TEM). The radiation response of the phosphates was evaluated by extracting the amorphous fraction at each irradiation fluence, and a single-impact model was used to determine the amorphous cross section and track diameter. Amorphization within individual ion tracks was confirmed using head-on TEM imaging, and the amorphous track size agreed with the value deduced by XRD analysis. Raman measurements were performed to qualitatively confirm the ion-induced crystalline-to-amorphous transformation which proceeds similarly for both phosphates. |
| 536 | _ | _ | |a 1411 - Nuclear Waste Disposal (POF4-141) |0 G:(DE-HGF)POF4-1411 |c POF4-141 |f POF IV |x 0 |
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| 700 | 1 | _ | |a Cooper, Jacob |0 P:(DE-HGF)0 |b 1 |
| 700 | 1 | _ | |a O'Quinn, Eric |0 P:(DE-HGF)0 |b 2 |
| 700 | 1 | _ | |a Cureton, William |0 P:(DE-HGF)0 |b 3 |
| 700 | 1 | _ | |a Palomares, Raul |0 P:(DE-HGF)0 |b 4 |
| 700 | 1 | _ | |a Leys, Julia |0 P:(DE-HGF)0 |b 5 |
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| 700 | 1 | _ | |a Neumeier, Stefan |0 P:(DE-Juel1)130389 |b 7 |
| 700 | 1 | _ | |a Chen, Chien-Hung |0 P:(DE-HGF)0 |b 8 |
| 700 | 1 | _ | |a Lang, Maik |0 P:(DE-HGF)0 |b 9 |e Corresponding author |
| 773 | _ | _ | |a 10.1016/j.nimb.2022.07.014 |g Vol. 527, p. 34 - 39 |0 PERI:(DE-600)1466524-4 |p 34 - 39 |t Nuclear instruments & methods in physics research / B |v 527 |y 2022 |x 0168-583X |
| 856 | 4 | _ | |u https://juser.fz-juelich.de/record/909075/files/Overstreet%20NIMB%202022.pdf |y Published on 2022-08-06. Available in OpenAccess from 2024-08-06. |
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| 913 | 1 | _ | |a DE-HGF |b Forschungsbereich Energie |l Nukleare Entsorgung, Sicherheit und Strahlenforschung (NUSAFE II) |1 G:(DE-HGF)POF4-140 |0 G:(DE-HGF)POF4-141 |3 G:(DE-HGF)POF4 |2 G:(DE-HGF)POF4-100 |4 G:(DE-HGF)POF |v Nukleare Entsorgung |9 G:(DE-HGF)POF4-1411 |x 0 |
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