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000909372 1001_ $$00000-0003-2440-6104$$aPozzer, Andrea$$b0$$eCorresponding author
000909372 245__ $$aSimulation of organics in the atmosphere: evaluation of EMACv2.54 with the Mainz Organic Mechanism (MOM) coupled to the ORACLE (v1.0) submodel
000909372 260__ $$aKatlenburg-Lindau$$bCopernicus$$c2022
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000909372 520__ $$aAn updated and expanded representation of organics in the chemistry general circulation model EMAC (ECHAM5/MESSy for Atmospheric Chemistry) has been evaluated. First, the comprehensive Mainz Organic Mechanism (MOM) in the submodel MECCA (Module Efficiently Calculating the Chemistry of the Atmosphere) was activated with explicit degradation of organic species up to five carbon atoms and a simplified mechanism for larger molecules. Second, the ORACLE submodel (version 1.0) now considers condensation on aerosols for all organics in the mechanism. Parameterizations for aerosol yields are used only for the lumped species that are not included in the explicit mechanism. The simultaneous usage of MOM and ORACLE allows an efficient estimation of not only the chemical degradation of the simulated volatile organic compounds but also the contribution of organics to the growth and fate of (organic) aerosol, with the complexity of the mechanism largely increased compared to EMAC simulations with more simplified chemistry. The model evaluation presented here reveals that the OH concentration is reproduced well globally, whereas significant biases for observed oxygenated organics are present. We also investigate the general properties of the aerosols and their composition, showing that the more sophisticated and process-oriented secondary aerosol formation does not degrade the good agreement of previous model configurations with observations at the surface, allowing further research in the field of gas–aerosol interactions.
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000909372 7001_ $$0P:(DE-HGF)0$$aReifenberg, Simon F.$$b1
000909372 7001_ $$00000-0002-8405-3470$$aKumar, Vinod$$b2
000909372 7001_ $$0P:(DE-Juel1)168550$$aFranco, Bruno$$b3
000909372 7001_ $$0P:(DE-HGF)0$$aKohl, Matthias$$b4
000909372 7001_ $$0P:(DE-Juel1)167439$$aTaraborrelli, Domenico$$b5
000909372 7001_ $$00000-0002-2542-3005$$aGromov, Sergey$$b6
000909372 7001_ $$00000-0002-6517-5341$$aEhrhart, Sebastian$$b7
000909372 7001_ $$0P:(DE-Juel1)188765$$aJöckel, Patrick$$b8
000909372 7001_ $$0P:(DE-Juel1)180928$$aSander, Rolf$$b9
000909372 7001_ $$0P:(DE-HGF)0$$aFall, Veronica$$b10
000909372 7001_ $$0P:(DE-Juel1)173788$$aRosanka, Simon$$b11
000909372 7001_ $$0P:(DE-Juel1)176592$$aKarydis, Vlassis$$b12
000909372 7001_ $$00000-0003-3104-5271$$aAkritidis, Dimitris$$b13
000909372 7001_ $$0P:(DE-Juel1)174161$$aEmmerichs, Tamara$$b14
000909372 7001_ $$0P:(DE-HGF)0$$aCrippa, Monica$$b15
000909372 7001_ $$0P:(DE-HGF)0$$aGuizzardi, Diego$$b16
000909372 7001_ $$00000-0003-3696-9123$$aKaiser, Johannes W.$$b17
000909372 7001_ $$00000-0002-8805-2141$$aClarisse, Lieven$$b18
000909372 7001_ $$0P:(DE-Juel1)4528$$aKiendler-Scharr, Astrid$$b19
000909372 7001_ $$00000-0002-3105-4306$$aTost, Holger$$b20
000909372 7001_ $$0P:(DE-Juel1)178035$$aTsimpidi, Alexandra$$b21$$ufzj
000909372 773__ $$0PERI:(DE-600)2456725-5$$a10.5194/gmd-15-2673-2022$$gVol. 15, no. 6, p. 2673 - 2710$$n6$$p2673 - 2710$$tGeoscientific model development$$v15$$x1991-959X$$y2022
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