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000909546 1001_ $$0P:(DE-HGF)0$$aWang, Jiqiang$$b0
000909546 245__ $$aFatigue-free artificial ionic skin toughened by self-healable elastic nanomesh
000909546 260__ $$a[London]$$bNature Publishing Group UK$$c2022
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000909546 520__ $$aRobust ionic sensing materials that are both fatigue-resistant and self-healable like human skin are essential for soft electronics and robotics with extended service life. However, most existing self-healable artificial ionic skins produced on the basis of network reconfiguration suffer from a low fatigue threshold due to the easy fracture of low-energy amorphous polymer chains with susceptible crack propagation. Here we engineer a fatigue-free yet fully healable hybrid ionic skin toughened by a high-energy, self-healable elastic nanomesh, resembling the repairable nanofibrous interwoven structure of human skin. Such a design affords a superhigh fatigue threshold of 2950 J m−2 while maintaining skin-like compliance, stretchability, and strain-adaptive stiffening response. Moreover, nanofiber tension-induced moisture breathing of ionic matrix leads to a record-high strain-sensing gauge factor of 66.8, far exceeding previous intrinsically stretchable ionic conductors. This concept creates opportunities for designing durable ion-conducting materials that replicate the unparalleled combinatory properties of natural skins more precisely
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000909546 65017 $$0V:(DE-MLZ)GC-1603-2016$$2V:(DE-HGF)$$aChemical Reactions and Advanced Materials$$x0
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000909546 7001_ $$0P:(DE-Juel1)151161$$aWu, Baohu$$b1$$ufzj
000909546 7001_ $$0P:(DE-HGF)0$$aWei, Peng$$b2
000909546 7001_ $$00000-0001-7471-686X$$aSun, Shengtong$$b3$$eCorresponding author
000909546 7001_ $$00000-0001-7235-210X$$aWu, Peiyi$$b4$$eCorresponding author
000909546 773__ $$0PERI:(DE-600)2553671-0$$a10.1038/s41467-022-32140-3$$gVol. 13, no. 1, p. 4411$$n1$$p4411$$tNature Communications$$v13$$x2041-1723$$y2022
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