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000909942 1001_ $$0P:(DE-HGF)0$$aKlein, J.$$b0$$eCorresponding author
000909942 245__ $$aControl of structure and spin texture in the van der Waals layered magnet CrSBr
000909942 260__ $$a[London]$$bNature Publishing Group UK$$c2022
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000909942 520__ $$aControlling magnetism at nanometer length scales is essential for realizing high-performance spintronic, magneto-electric and topological devices and creating on-demand spin Hamiltonians probing fundamental concepts in physics. Van der Waals (vdW)-bonded layered magnets offer exceptional opportunities for such spin texture engineering. Here, we demonstrate nanoscale structural control in the layered magnet CrSBr with the potential to create spin patterns without the environmental sensitivity that has hindered such manipulations in other vdW magnets. We drive a local phase transformation using an electron beam that moves atoms and exchanges bond directions, effectively creating regions that have vertical vdW layers embedded within the initial horizontally vdW bonded exfoliated flakes. We calculate that the newly formed two-dimensional structure is ferromagnetically ordered in-plane with an energy gap in the visible spectrum, and weak antiferromagnetism between the planes, suggesting possibilities for creating spin textures and quantum magnetic phases.
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000909942 536__ $$0G:(EU-Grant)856538$$a3D MAGiC - Three-dimensional magnetization textures: Discovery and control on the nanoscale (856538)$$c856538$$fERC-2019-SyG$$x1
000909942 536__ $$0G:(EU-Grant)823717$$aESTEEM3 - Enabling Science and Technology through European Electron Microscopy (823717)$$c823717$$fH2020-INFRAIA-2018-1$$x2
000909942 536__ $$0G:(GEPRIS)405553726$$aDFG project 405553726 - TRR 270: Hysterese-Design magnetischer Materialien für effiziente Energieumwandlung (405553726)$$c405553726$$x3
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000909942 7001_ $$0P:(DE-HGF)0$$aPham, T.$$b1
000909942 7001_ $$0P:(DE-HGF)0$$aThomsen, J. D.$$b2
000909942 7001_ $$00000-0001-8544-0555$$aCurtis, J. B.$$b3
000909942 7001_ $$0P:(DE-Juel1)172928$$aDenneulin, T.$$b4
000909942 7001_ $$0P:(DE-Juel1)132889$$aLorke, M.$$b5$$ufzj
000909942 7001_ $$0P:(DE-HGF)0$$aFlorian, M.$$b6
000909942 7001_ $$00000-0002-8134-4344$$aSteinhoff, A.$$b7
000909942 7001_ $$0P:(DE-HGF)0$$aWiscons, R. A.$$b8
000909942 7001_ $$0P:(DE-HGF)0$$aLuxa, J.$$b9
000909942 7001_ $$0P:(DE-HGF)0$$aSofer, Z.$$b10
000909942 7001_ $$0P:(DE-Juel1)129336$$aJahnke, F.$$b11$$ufzj
000909942 7001_ $$00000-0003-3956-4594$$aNarang, P.$$b12$$eCorresponding author
000909942 7001_ $$00000-0003-0838-9770$$aRoss, F. M.$$b13$$eCorresponding author
000909942 773__ $$0PERI:(DE-600)2553671-0$$a10.1038/s41467-022-32737-8$$gVol. 13, no. 1, p. 5420$$n1$$p5420$$tNature Communications$$v13$$x2041-1723$$y2022
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