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@ARTICLE{Klein:909942,
author = {Klein, J. and Pham, T. and Thomsen, J. D. and Curtis, J. B.
and Denneulin, T. and Lorke, M. and Florian, M. and
Steinhoff, A. and Wiscons, R. A. and Luxa, J. and Sofer, Z.
and Jahnke, F. and Narang, P. and Ross, F. M.},
title = {{C}ontrol of structure and spin texture in the van der
{W}aals layered magnet {C}r{SB}r},
journal = {Nature Communications},
volume = {13},
number = {1},
issn = {2041-1723},
address = {[London]},
publisher = {Nature Publishing Group UK},
reportid = {FZJ-2022-03536},
pages = {5420},
year = {2022},
abstract = {Controlling magnetism at nanometer length scales is
essential for realizing high-performance spintronic,
magneto-electric and topological devices and creating
on-demand spin Hamiltonians probing fundamental concepts in
physics. Van der Waals (vdW)-bonded layered magnets offer
exceptional opportunities for such spin texture engineering.
Here, we demonstrate nanoscale structural control in the
layered magnet CrSBr with the potential to create spin
patterns without the environmental sensitivity that has
hindered such manipulations in other vdW magnets. We drive a
local phase transformation using an electron beam that moves
atoms and exchanges bond directions, effectively creating
regions that have vertical vdW layers embedded within the
initial horizontally vdW bonded exfoliated flakes. We
calculate that the newly formed two-dimensional structure is
ferromagnetically ordered in-plane with an energy gap in the
visible spectrum, and weak antiferromagnetism between the
planes, suggesting possibilities for creating spin textures
and quantum magnetic phases.},
cin = {ER-C-1},
ddc = {500},
cid = {I:(DE-Juel1)ER-C-1-20170209},
pnm = {5351 - Platform for Correlative, In Situ and Operando
Characterization (POF4-535) / 3D MAGiC - Three-dimensional
magnetization textures: Discovery and control on the
nanoscale (856538) / ESTEEM3 - Enabling Science and
Technology through European Electron Microscopy (823717) /
DFG project 405553726 - TRR 270: Hysterese-Design
magnetischer Materialien für effiziente Energieumwandlung
(405553726)},
pid = {G:(DE-HGF)POF4-5351 / G:(EU-Grant)856538 /
G:(EU-Grant)823717 / G:(GEPRIS)405553726},
typ = {PUB:(DE-HGF)16},
pubmed = {36109520},
UT = {WOS:000854795700015},
doi = {10.1038/s41467-022-32737-8},
url = {https://juser.fz-juelich.de/record/909942},
}