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@ARTICLE{Vojtech:910024,
author = {Vojtech, V. and Charilaou, M. and Kovács, A. and Firlus,
A. and Gerstl, S. S. A. and Dunin-Borkowski, R. E. and
Löffler, J. F. and Schäublin, R. E.},
title = {{M}acroscopic magnetic hardening due to nanoscale spinodal
decomposition in {F}e–{C}r},
journal = {Acta materialia},
volume = {240},
issn = {1359-6454},
address = {Amsterdam [u.a.]},
publisher = {Elsevier Science},
reportid = {FZJ-2022-03579},
pages = {118265 -},
year = {2022},
abstract = {The Fe–Cr alloy system is the basis of ferritic steels,
which are important structural materials for many
applications, including their use in future fusion reactors.
However, when exposed to elevated temperatures and
radiation, the Fe–Cr system can undergo phase separation,
resulting in Fe-rich (α) and Cr-rich (α’) nanoscale
regions. This in turn generates the so-called “475 °C
embrittlement” and modifies the magnetic properties. The
correlation between the microstructural and magnetic changes
is however poorly understood, which currently prevents the
possibility of assessing the material in a non-destructive
way by magnetometry. Here, we study the microstructural
decomposition of an Fe–40Cr alloy induced by annealing at
500 °C for extensive time scales and its impact on the
magnetic properties using magnetometry and advanced
experimental methods, such as atom probe tomography,
transmission electron microscopy (TEM), and micromagnetic
simulations. Upon annealing, the alloy rapidly exhibits a
spinodal decomposition morphology with a typical length
scale of about 10 nm. With increasing annealing time, the
hardness assessed by Vickers testing, the magnetic
saturation, and the coercivity increase, which correlates
with an increase in α-volume fraction and the system's
heterogeneity. The magnetic domain patterns imaged by TEM
and interpreted with the help of micromagnetic simulations
reveal at the nanometer scale the impact of decomposition on
the magnetic response of Fe–Cr.},
cin = {ER-C-1},
ddc = {670},
cid = {I:(DE-Juel1)ER-C-1-20170209},
pnm = {5351 - Platform for Correlative, In Situ and Operando
Characterization (POF4-535) / DFG project 405553726 - TRR
270: Hysterese-Design magnetischer Materialien für
effiziente Energieumwandlung (405553726) / 3D MAGiC -
Three-dimensional magnetization textures: Discovery and
control on the nanoscale (856538)},
pid = {G:(DE-HGF)POF4-5351 / G:(GEPRIS)405553726 /
G:(EU-Grant)856538},
typ = {PUB:(DE-HGF)16},
UT = {WOS:000862266600001},
doi = {10.1016/j.actamat.2022.118265},
url = {https://juser.fz-juelich.de/record/910024},
}