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000910170 1001_ $$0P:(DE-Juel1)176115$$aVerlinden, Bart$$b0$$eCorresponding author
000910170 245__ $$aSolvent Optimization Studies for a New EURO-GANEX Process with 2,2’-Oxybis( N,N -di- n -decylpropanamide) (mTDDGA) and Its Radiolysis Products
000910170 260__ $$aPhiladelphia, PA$$bTaylor & Francis$$c2023
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000910170 520__ $$aThe diglycolamide 2,2'-oxybis(N,N-di-n-decylpropanamide) (mTDDGA) is studied as an extractant for actinides and lanthanides in the European Grouped Actinide Extraction (EURO-GANEX) process, aiming at a more simplified process suing a single extractant instead of a mixture of extractants used in the current EURO-GANEX process. This study presents solvent optimization studies of mTDDGA, with regards to the extraction characteristics of the different diastereomers, Pu loading capacity after gamma-irradiation of the solvent up to 445 kGy, quantification of degradation compounds and extraction characteristic of the degradation compounds themselves. Like other methylated diglycolamides, we found a remarkable difference in extraction of up to two orders of magnitudes between the two diastereomers. High Pu loading (36 g L-1) is feasible using this single extractant, even after absorbing 445 kGy, possibly promoted by the presence of the main degradation compound which extracts Pu very well.
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000910170 7001_ $$0P:(DE-Juel1)130438$$aWilden, Andreas$$b1
000910170 7001_ $$00000-0002-7100-192X$$aVan Hecke, Karen$$b2
000910170 7001_ $$00000-0002-2505-9960$$aJ. M. Egberink, Richard$$b3
000910170 7001_ $$00000-0002-4596-9179$$aHuskens, Jurriaan$$b4
000910170 7001_ $$00000-0002-6863-8655$$aVerboom, Willem$$b5
000910170 7001_ $$0P:(DE-Juel1)142389$$aHupert, Michelle$$b6
000910170 7001_ $$aWeßling, Patrik$$b7
000910170 7001_ $$00000-0003-1436-8247$$aGeist, Andreas$$b8
000910170 7001_ $$aPanak, Petra J.$$b9
000910170 7001_ $$aHermans, Rainier$$b10
000910170 7001_ $$00000-0002-2385-6093$$aVerwerft, Marc$$b11
000910170 7001_ $$0P:(DE-Juel1)130383$$aModolo, Giuseppe$$b12
000910170 7001_ $$00000-0003-4768-3606$$aBinnemans, Koen$$b13
000910170 7001_ $$00000-0002-2695-1002$$aCardinaels, Thomas$$b14
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