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@ARTICLE{Verlinden:910170,
      author       = {Verlinden, Bart and Wilden, Andreas and Van Hecke, Karen
                      and J. M. Egberink, Richard and Huskens, Jurriaan and
                      Verboom, Willem and Hupert, Michelle and Weßling, Patrik
                      and Geist, Andreas and Panak, Petra J. and Hermans, Rainier
                      and Verwerft, Marc and Modolo, Giuseppe and Binnemans, Koen
                      and Cardinaels, Thomas},
      title        = {{S}olvent {O}ptimization {S}tudies for a {N}ew
                      {EURO}-{GANEX} {P}rocess with 2,2’-{O}xybis( {N},{N} -di-
                      n -decylpropanamide) (m{TDDGA}) and {I}ts {R}adiolysis
                      {P}roducts},
      journal      = {Solvent extraction and ion exchange},
      volume       = {41},
      number       = {1},
      issn         = {0736-6299},
      address      = {Philadelphia, PA},
      publisher    = {Taylor $\&$ Francis},
      reportid     = {FZJ-2022-03652},
      pages        = {59-87},
      year         = {2023},
      abstract     = {The diglycolamide 2,2'-oxybis(N,N-di-n-decylpropanamide)
                      (mTDDGA) is studied as an extractant for actinides and
                      lanthanides in the European Grouped Actinide Extraction
                      (EURO-GANEX) process, aiming at a more simplified process
                      suing a single extractant instead of a mixture of
                      extractants used in the current EURO-GANEX process. This
                      study presents solvent optimization studies of mTDDGA, with
                      regards to the extraction characteristics of the different
                      diastereomers, Pu loading capacity after gamma-irradiation
                      of the solvent up to 445 kGy, quantification of degradation
                      compounds and extraction characteristic of the degradation
                      compounds themselves. Like other methylated diglycolamides,
                      we found a remarkable difference in extraction of up to two
                      orders of magnitudes between the two diastereomers. High Pu
                      loading (36 g L-1) is feasible using this single extractant,
                      even after absorbing 445 kGy, possibly promoted by the
                      presence of the main degradation compound which extracts Pu
                      very well.},
      cin          = {IEK-6 / ZEA-3},
      ddc          = {540},
      cid          = {I:(DE-Juel1)IEK-6-20101013 / I:(DE-Juel1)ZEA-3-20090406},
      pnm          = {1412 - Predisposal (POF4-141) / GENIORS - GEN IV Integrated
                      Oxide fuels recycling strategies (755171)},
      pid          = {G:(DE-HGF)POF4-1412 / G:(EU-Grant)755171},
      typ          = {PUB:(DE-HGF)16},
      UT           = {WOS:000863644600001},
      doi          = {10.1080/07366299.2022.2125151},
      url          = {https://juser.fz-juelich.de/record/910170},
}