Home > Publications database > Solvent Optimization Studies for a New EURO-GANEX Process with 2,2’-Oxybis( N,N -di- n -decylpropanamide) (mTDDGA) and Its Radiolysis Products > print

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005     20240712084604.0
024 7 _ |a 10.1080/07366299.2022.2125151
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024 7 _ |a 1532-2262
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100 1 _ |a Verlinden, Bart
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245 _ _ |a Solvent Optimization Studies for a New EURO-GANEX Process with 2,2’-Oxybis( N,N -di- n -decylpropanamide) (mTDDGA) and Its Radiolysis Products
260 _ _ |a Philadelphia, PA
|c 2023
|b Taylor & Francis
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520 _ _ |a The diglycolamide 2,2'-oxybis(N,N-di-n-decylpropanamide) (mTDDGA) is studied as an extractant for actinides and lanthanides in the European Grouped Actinide Extraction (EURO-GANEX) process, aiming at a more simplified process suing a single extractant instead of a mixture of extractants used in the current EURO-GANEX process. This study presents solvent optimization studies of mTDDGA, with regards to the extraction characteristics of the different diastereomers, Pu loading capacity after gamma-irradiation of the solvent up to 445 kGy, quantification of degradation compounds and extraction characteristic of the degradation compounds themselves. Like other methylated diglycolamides, we found a remarkable difference in extraction of up to two orders of magnitudes between the two diastereomers. High Pu loading (36 g L-1) is feasible using this single extractant, even after absorbing 445 kGy, possibly promoted by the presence of the main degradation compound which extracts Pu very well.
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700 1 _ |a Wilden, Andreas
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700 1 _ |a Van Hecke, Karen
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700 1 _ |a J. M. Egberink, Richard
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700 1 _ |a Huskens, Jurriaan
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700 1 _ |a Verboom, Willem
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700 1 _ |a Hupert, Michelle
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700 1 _ |a Weßling, Patrik
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700 1 _ |a Geist, Andreas
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700 1 _ |a Panak, Petra J.
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700 1 _ |a Hermans, Rainier
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700 1 _ |a Verwerft, Marc
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700 1 _ |a Modolo, Giuseppe
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700 1 _ |a Binnemans, Koen
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700 1 _ |a Cardinaels, Thomas
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773 _ _ |a 10.1080/07366299.2022.2125151
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|t Solvent extraction and ion exchange
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