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@ARTICLE{Roy:910213,
author = {Roy, Shyamal and Prakash, A. and Sandfeld, S.},
title = {{S}intering of alumina nanoparticles: comparison of
interatomic potentials, molecular dynamics simulations, and
data analysis},
journal = {Modelling and simulation in materials science and
engineering},
volume = {30},
number = {6},
issn = {0965-0393},
address = {Bristol},
publisher = {IOP Publ.},
reportid = {FZJ-2022-03690},
pages = {065009 -},
year = {2022},
abstract = {Sintering of alumina nanoparticles is of interest both from
the view of fundamental research as well as for industrial
applications. Atomistic simulations are tailor-made for
understanding and predicting the time- and
temperature-dependent sintering behaviour. However, the
quality and predictability of such analysis is strongly
dependent on the performance of the underlying interatomic
potentials. In this work, we investigate and benchmark four
empirical interatomic potentials and discuss the resulting
properties and drawbacks based on experimental and density
functional theory data from the literature. The potentials,
which have different origins and formulations, are then used
in molecular dynamics (MD) simulations to perform a
systematic study of the sintering process. To analyse the
results, we develop a number of tailored data analysis
approaches that are able to characterise and quantify the
sintering process. Subsequently, the disparities in the
sintering behaviour predicted by the potentials are
critically discussed. Finally, we conclude by providing
explanations for the differences in performance of the
potentials, together with recommendations for MD sintering
simulations of alumina.},
cin = {IAS-9},
ddc = {530},
cid = {I:(DE-Juel1)IAS-9-20201008},
pnm = {5111 - Domain-Specific Simulation $\&$ Data Life Cycle Labs
(SDLs) and Research Groups (POF4-511)},
pid = {G:(DE-HGF)POF4-5111},
typ = {PUB:(DE-HGF)16},
UT = {WOS:000840970100001},
doi = {10.1088/1361-651X/ac8172},
url = {https://juser.fz-juelich.de/record/910213},
}