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@ARTICLE{Yuan:910218,
      author       = {Yuan, Ye and Yan, Genghua and Hong, Ruijiang and Liang,
                      Zongcun and Kirchartz, Thomas},
      title        = {{Q}uantifying {E}fficiency {L}imitations in
                      {A}ll‐{I}norganic {H}alide {P}erovskite {S}olar {C}ells},
      journal      = {Advanced materials},
      volume       = {34},
      number       = {21},
      issn         = {0935-9648},
      address      = {Weinheim},
      publisher    = {Wiley-VCH},
      reportid     = {FZJ-2022-03695},
      pages        = {210813},
      year         = {2022},
      abstract     = {While halide perovskites have excellent optoelectronic
                      properties, their poor stability is a major obstacle toward
                      commercialization. There is a strong interest to move away
                      from organic A-site cations such as methylammonium and
                      formamidinium toward Cs with the aim of improving thermal
                      stability of the perovskite layers. While the optoelectronic
                      properties and the device performance of Cs-based
                      all-inorganic lead-halide perovskites are very good, they
                      are still trailing behind those of perovskites that use
                      organic cations. Here, the state-of-the-art of all-inorganic
                      perovskites for photovoltaic applications is reviewed by
                      performing detailed meta-analyses of key performance
                      parameters on the cell and material level. Key material
                      properties such as carrier mobilities, external
                      photoluminescence quantum efficiency, and photoluminescence
                      lifetime are discussed and what is known about defect
                      tolerance in all-inorganic is compared relative to hybrid
                      (organic–inorganic) perovskites. Subsequently, a unified
                      approach is adopted for analyzing performance losses in
                      perovskite solar cells based on breaking down the losses
                      into several figures of merit representing recombination
                      losses, resistive losses, and optical losses. Based on this
                      detailed loss analysis, guidelines are eventually developed
                      for future performance improvement of all-inorganic
                      perovskite solar cells.},
      cin          = {IEK-5},
      ddc          = {660},
      cid          = {I:(DE-Juel1)IEK-5-20101013},
      pnm          = {1213 - Cell Design and Development (POF4-121)},
      pid          = {G:(DE-HGF)POF4-1213},
      typ          = {PUB:(DE-HGF)16},
      pubmed       = {35014106},
      UT           = {WOS:000773570300001},
      doi          = {10.1002/adma.202108132},
      url          = {https://juser.fz-juelich.de/record/910218},
}