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000910298 1001_ $$0P:(DE-HGF)0$$aKarasahin, Aziz$$b0$$eCorresponding author
000910298 245__ $$aSingle quantum emitters with spin ground states based on Cl bound excitons in ZnSe
000910298 260__ $$aWoodbury, NY$$bInst.$$c2022
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000910298 520__ $$aDefects in wide-band-gap semiconductors are promising qubit candidates for quantum communication and computation. Epitaxially grown II-VI semiconductors are particularly promising host materials due to their direct band gap and potential for isotopic purification to a spin-zero nuclear background. Here, we show an alternative type of single photon emitter with potential electron spin qubits based on Cl impurities in ZnSe. We utilize a quantum well to increase the binding energies of donor emission and confirm single photon emission with short radiative lifetimes of 192 ps. Furthermore, we verify that the ground state of the Cl donor complex contains a single electron by observing two-electron-satellite emission, leaving the electron in higher orbital states. We also characterize the Zeeman splitting of the exciton transition by performing polarization-resolved magnetic spectroscopy on single emitters. Our results suggest single Cl impurities are suitable as a single photon source with a potential photonic interface.
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000910298 536__ $$0G:(GEPRIS)337456818$$aDFG project 337456818 - Entwicklung von Spin-Qubit Bauelementen aus ZnSe/$$c337456818$$x1
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000910298 7001_ $$0P:(DE-HGF)0$$aPettit, Robert M.$$b1
000910298 7001_ $$0P:(DE-Juel1)161247$$avon den Driesch, Nils$$b2
000910298 7001_ $$0P:(DE-HGF)0$$aJansen, Marvin Marco$$b3
000910298 7001_ $$0P:(DE-Juel1)166158$$aPawlis, Alexander$$b4
000910298 7001_ $$0P:(DE-HGF)0$$aWaks, Edo$$b5
000910298 773__ $$0PERI:(DE-600)2844156-4$$a10.1103/PhysRevA.106.L030402$$gVol. 106, no. 3, p. L030402$$n3$$pL030402$$tPhysical review / A$$v106$$x2469-9926$$y2022
000910298 8564_ $$uhttps://juser.fz-juelich.de/record/910298/files/PhysRevA.106.L030402.pdf$$yOpenAccess
000910298 8564_ $$uhttps://juser.fz-juelich.de/record/910298/files/Preprint_2_Manuscript-Cl_BoundExcitons.pdf$$yOpenAccess
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