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000009107 0247_ $$2DOI$$a10.1016/j.progsolidstchem.2009.11.004
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000009107 084__ $$2WoS$$aChemistry, Inorganic & Nuclear
000009107 1001_ $$0P:(DE-HGF)0$$aLerch, M.$$b0
000009107 245__ $$aOxide nitrides: From oxides to solids with mobile nitrogen ions
000009107 260__ $$aOxford [u.a.]$$bPergamon Press$$c2009
000009107 300__ $$a
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000009107 440_0 $$010541$$aProgress in Solid State Chemistry$$v37$$x0079-6786$$y2
000009107 500__ $$aThis work has been funded by the DFG in the frame of the priority program 1136 'Substitutional effects in ionic solids'.
000009107 520__ $$aThe possibility of fast nitrogen ion conduction in solids is reviewed. Promising electrolytes based on three different base compounds are in the focus of this contribution: Zirconium oxide nitrides, tantalum oxide nitrides and mayenite-based materials. All aspects ranging from preparation methods, crystal structures (ideal and defect structure, also at elevated temperatures), transport properties (ionic and electronic conductivity, transference numbers, diffusion) and correlations between structure and physical properties are presented and discussed, in part also in relation to theoretical calculations. Fluorite-type quaternary oxide nitrides of zirconium are proven to be the first known materials with high nitrogen ion mobility. They can be described as fast mixed oxygen/nitrogen conductors but are limited due to the low maximum nitrogen/oxygen ratio achievable. Corresponding phases based on stabilized tantalum oxide nitrides have a superior N/O ratio but show poor thermal stability. For the development of a pure nitrogen ion conductor a different approach has also been investigated: Some cage compounds, in particular mayenite, allow the substitution of oxygen anions not tightly bound in the framework by nitrogen ions. Some of the obtained N-containing phases exhibit an outstanding electrical conductivity at low temperatures. Possible devices and applications such as a new type of a nitrogen sensor and an ammonia-producing fuel cell are introduced and discussed. (C) 2009 Elsevier Ltd. All rights reserved.
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000009107 65320 $$2Author$$aSolid electrolytes
000009107 65320 $$2Author$$aMobile nitrogen ions
000009107 65320 $$2Author$$aOxide nitrides.
000009107 65320 $$2Author$$aTransport properties
000009107 65320 $$2Author$$aCorrelations between crystal structure and physical properties
000009107 7001_ $$0P:(DE-HGF)0$$aJanek, J.$$b1
000009107 7001_ $$0P:(DE-HGF)0$$aBecker, K.D.$$b2
000009107 7001_ $$0P:(DE-HGF)0$$aBerendts, S.$$b3
000009107 7001_ $$0P:(DE-HGF)0$$aBoysen, H.$$b4
000009107 7001_ $$0P:(DE-HGF)0$$aBredow, T.$$b5
000009107 7001_ $$0P:(DE-HGF)0$$aDronskowski, R.$$b6
000009107 7001_ $$0P:(DE-HGF)0$$aEgginghaus, S.G.$$b7
000009107 7001_ $$0P:(DE-HGF)0$$aKilo, M.$$b8
000009107 7001_ $$0P:(DE-Juel1)VDB91181$$aLumey, M.W.$$b9$$uFZJ
000009107 7001_ $$0P:(DE-HGF)0$$aMartin, M.$$b10
000009107 7001_ $$0P:(DE-HGF)0$$aReimann, C.$$b11
000009107 7001_ $$0P:(DE-HGF)0$$aSchweda, E.$$b12
000009107 7001_ $$0P:(DE-Juel1)VDB85752$$aValov, I.$$b13$$uFZJ
000009107 7001_ $$0P:(DE-HGF)0$$aWiemhöfer, H.D.$$b14
000009107 773__ $$0PERI:(DE-600)2013358-3$$a10.1016/j.progsolidstchem.2009.11.004$$gVol. 37$$q37$$tProgress in solid state chemistry$$v37$$x0079-6786$$y2009
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