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@ARTICLE{Tas:910786,
author = {Tas, M. and Şaşıoğlu, E. and Blügel, S. and Mertig, I.
and Galanakis, I.},
title = {{A}b initio calculation of the {H}ubbard {U} and {H}und
exchange {J} in local moment magnets: {T}he case of
{M}n-based full {H}eusler compounds},
journal = {Physical review materials},
volume = {6},
number = {11},
issn = {2475-9953},
address = {College Park, MD},
publisher = {APS},
reportid = {FZJ-2022-04138},
pages = {114401},
year = {2022},
abstract = {Mn-based full Heusler compounds possess well-defined local
atomic Mn moments, and thus the correlation effects between
localized d electrons are expected to play an important role
in determining the electronic and magnetic properties of
these materials. Employing ab initio calculations in
conjunction with the constrained random-phase approximation
(cRPA) method, we calculate the strength of the effective
on-site Coulomb interaction parameters (Hubbard U and Hund
exchange J) in the case of X2MnZ full Heusler compounds with
X being one of Ni, Pd, or Cu, and Z being one of In, Sn, Sb,
or Te. We show that the Z element (or sp element) in Heusler
compounds significantly reduces the strength of the Hubbard
U parameter for Mn 3d electrons compared to the elementary
bulk Mn. On the contrary, the effect of the sp atom on the
strength of the U parameter of Ni, Cu, or Pd valence d
electrons is not so substantial with respect to the
elementary bulk values. The U values for all
transition-metal atoms decrease with increasing sp electron
numbers in the In-Sn-Sb-Te sequence. Our cRPA calculations
reveal that despite their well-defined local magnetic
moments, the Mn-based full Heusler alloys fall into the
category of the weakly correlated materials.},
cin = {IAS-1 / PGI-1 / JARA-FIT / JARA-HPC},
ddc = {530},
cid = {I:(DE-Juel1)IAS-1-20090406 / I:(DE-Juel1)PGI-1-20110106 /
$I:(DE-82)080009_20140620$ / $I:(DE-82)080012_20140620$},
pnm = {5211 - Topological Matter (POF4-521)},
pid = {G:(DE-HGF)POF4-5211},
typ = {PUB:(DE-HGF)16},
UT = {WOS:000884781000003},
doi = {10.1103/PhysRevMaterials.6.114401},
url = {https://juser.fz-juelich.de/record/910786},
}